Literature DB >> 31922852

Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe_{3}Sb[Pd(dmit)_{2}]_{2}.

J M Ni1, B L Pan1, B Q Song1, Y Y Huang1, J Y Zeng1, Y J Yu1, E J Cheng1, L S Wang1, D Z Dai1, R Kato2, S Y Li1,3.   

Abstract

We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe_{3}Sb[Pd(dmit)_{2}]_{2}, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)NCAOBW2041-172310.1038/ncomms1274]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe_{3}Sb[Pd(dmit)_{2}]_{2} [M. Yamashita et al., Science 328, 1246 (2010)SCIEAS0036-807510.1126/science.1188200], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe_{3}Sb[Pd(dmit)_{2}]_{2} has to be reconsidered.

Entities:  

Year:  2019        PMID: 31922852     DOI: 10.1103/PhysRevLett.123.247204

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  3 in total

1.  Resistivity and thermal conductivity of an organic insulator β'-EtMe3Sb[Pd(dmit)2]2.

Authors:  Minoru Yamashita; Yuki Sato; Yuichi Kasahara; Shigeru Kasahara; Takasada Shibauchi; Yuji Matsuda
Journal:  Sci Rep       Date:  2022-06-02       Impact factor: 4.996

2.  Giant isotropic magneto-thermal conductivity of metallic spin liquid candidate Pr2Ir2O7 with quantum criticality.

Authors:  J M Ni; Y Y Huang; E J Cheng; Y J Yu; B L Pan; Q Li; L M Xu; Z M Tian; S Y Li
Journal:  Nat Commun       Date:  2021-01-12       Impact factor: 14.919

3.  Charge-neutral fermions and magnetic field-driven instability in insulating YbIr3Si7.

Authors:  Y Sato; S Suetsugu; T Tominaga; Y Kasahara; S Kasahara; T Kobayashi; S Kitagawa; K Ishida; R Peters; T Shibauchi; A H Nevidomskyy; L Qian; E Morosan; Y Matsuda
Journal:  Nat Commun       Date:  2022-01-19       Impact factor: 14.919

  3 in total

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