Literature DB >> 31503495

Frequency-, Time-, and Wavevector-Resolved Ultrafast Incoherent Diffraction of Noisy X-ray Pulses.

Shahaf Asban1, Daeheum Cho1, Shaul Mukamel1.   

Abstract

We study theoretically incoherent time-resolved X-ray diffraction of fluctuating sources such as free electron lasers, as well as coherent sources with controllably added randomness. We find that the temporal resolution is strongly eroded by the noise. By considering frequency resolution of the signal, we find that the statistical properties of the noise carry important information allowing us to restore the temporal resolution. We propose a multidimensional stochastic resonance treatment to shape the optical window and extract this information from signals. Using the frequency-dependent stochastic phase as a frequency marker allows to improve the spectral resolution as well via intensity correlations. Frequency-tuned field correlation functions are used to modify the effective frequency gating and extract specific charge density contributions to the diffraction pattern while maintaining temporal resolution.

Entities:  

Year:  2019        PMID: 31503495     DOI: 10.1021/acs.jpclett.9b00924

Source DB:  PubMed          Journal:  J Phys Chem Lett        ISSN: 1948-7185            Impact factor:   6.475


  5 in total

1.  Unveiling the spatial distribution of molecular coherences at conical intersections by covariance X-ray diffraction signals.

Authors:  Stefano M Cavaletto; Daniel Keefer; Jérémy R Rouxel; Flavia Aleotti; Francesco Segatta; Marco Garavelli; Shaul Mukamel
Journal:  Proc Natl Acad Sci U S A       Date:  2021-06-01       Impact factor: 11.205

2.  Sensing ultrashort electronic coherent beating at conical intersections by single-electron pulses.

Authors:  Shahaf Asban; Daniel Keefer; Vladimir Y Chernyak; Shaul Mukamel
Journal:  Proc Natl Acad Sci U S A       Date:  2022-05-24       Impact factor: 12.779

3.  Signatures of electronic and nuclear coherences in ultrafast molecular x-ray and electron diffraction.

Authors:  Jérémy R Rouxel; Daniel Keefer; Shaul Mukamel
Journal:  Struct Dyn       Date:  2021-01-11       Impact factor: 2.920

4.  Transient measurement of phononic states with covariance-based stochastic spectroscopy.

Authors:  Giorgia Sparapassi; Stefano M Cavaletto; Jonathan Tollerud; Angela Montanaro; Filippo Glerean; Alexandre Marciniak; Fancesca Giusti; Shaul Mukamel; Daniele Fausti
Journal:  Light Sci Appl       Date:  2022-03-01       Impact factor: 17.782

5.  Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser.

Authors:  Franklin D Fuller; Anton Loukianov; Tsukasa Takanashi; Daehyun You; Yiwen Li; Kiyoshi Ueda; Thomas Fransson; Makina Yabashi; Tetsuo Katayama; Tsu-Chien Weng; Roberto Alonso-Mori; Uwe Bergmann; Jan Kern; Vittal K Yachandra; Philippe Wernet; Junko Yano
Journal:  Commun Chem       Date:  2021-06-07
  5 in total

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