Literature DB >> 31123131

Electrified methane reforming: A compact approach to greener industrial hydrogen production.

Sebastian T Wismann1, Jakob S Engbæk2, Søren B Vendelbo2, Flemming B Bendixen3, Winnie L Eriksen4, Kim Aasberg-Petersen4, Cathrine Frandsen1, Ib Chorkendorff5, Peter M Mortensen6.   

Abstract

Electrification of conventionally fired chemical reactors has the potential to reduce CO2 emissions and provide flexible and compact heat generation. Here, we describe a disruptive approach to a fundamental process by integrating an electrically heated catalytic structure directly into a steam-methane-reforming (SMR) reactor for hydrogen production. Intimate contact between the electric heat source and the reaction site drives the reaction close to thermal equilibrium, increases catalyst utilization, and limits unwanted byproduct formation. The integrated design with small characteristic length scales allows compact reactor designs, potentially 100 times smaller than current reformer platforms. Electrification of SMR offers a strong platform for new reactor design, scale, and implementation opportunities. Implemented on a global scale, this could correspond to a reduction of nearly 1% of all CO2 emissions.
Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

Entities:  

Year:  2019        PMID: 31123131     DOI: 10.1126/science.aaw8775

Source DB:  PubMed          Journal:  Science        ISSN: 0036-8075            Impact factor:   47.728


  4 in total

1.  Technoeconomic Evaluation of the Industrial Implementation of Catalytic Direct Nonoxidative Methane Coupling.

Authors:  Rolf S Postma; Dylan J Keijsper; Bart F Morsink; Erwin H Siegers; Muhammed E E Mercimek; Lance K Nieukoop; Henk van den Berg; Aloijsius G J van der Ham; Leon Lefferts
Journal:  Ind Eng Chem Res       Date:  2021-12-15       Impact factor: 3.720

2.  Catalytic production of low-carbon footprint sustainable natural gas.

Authors:  Xiaoqin Si; Rui Lu; Zhitong Zhao; Xiaofeng Yang; Feng Wang; Huifang Jiang; Xiaolin Luo; Aiqin Wang; Zhaochi Feng; Jie Xu; Fang Lu
Journal:  Nat Commun       Date:  2022-01-11       Impact factor: 14.919

3.  Supra Hydrolytic Catalysis of Ni3 Fe/rGO for Hydrogen Generation.

Authors:  Jiangchuan Liu; Mengchen Zhang; Qinke Tang; Yingyan Zhao; Jiguang Zhang; Yunfeng Zhu; Yana Liu; Xiaohui Hu; Liquan Li
Journal:  Adv Sci (Weinh)       Date:  2022-05-06       Impact factor: 17.521

4.  Electrosynthesis of ammonia with high selectivity and high rates via engineering of the solid-electrolyte interphase.

Authors:  Shaofeng Li; Yuanyuan Zhou; Katja Li; Mattia Saccoccio; Rokas Sažinas; Suzanne Z Andersen; Jakob B Pedersen; Xianbiao Fu; Vahid Shadravan; Debasish Chakraborty; Jakob Kibsgaard; Peter C K Vesborg; Jens K Nørskov; Ib Chorkendorff
Journal:  Joule       Date:  2022-09-21
  4 in total

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