| Literature DB >> 30960714 |
Shuming Chen1, Wenbo Zhu2, Yabing Cheng3.
Abstract
Polyurethane (PU) foams are widely used as acoustic package materials to eliminate vehicle interior noise. Therefore, it is important to improve the acoustic performances of PU foams. In this paper, the grey relational analysis (GRA) method and multi-objective particle swarm optimization (MOPSO) algorithm are applied to improve the acoustic performances of PU foam composites. The average sound absorption coefficient and average transmission loss are set as optimization objectives. The hardness and content of Ethylene Propylene Diene Monomer (EPDM) and the content of deionized water and modified isocyanate (MDI) are selected as design variables. The optimization process of GRA method is based on the orthogonal arrays L9(34), and the MOPSO algorithm is based on the Response Surface (RS) surrogate model. The results show that the acoustic performances of PU foam composites can be improved by optimizing the synthetic formula. Meanwhile, the results that were obtained by GRA method show the degree of influence of the four design variables on the optimization objectives, and the results obtained by MOPSO algorithm show the specific effects of the four design variables on the optimization objectives. Moreover, according to the confirmation experiment, the optimal synthetic formula is obtained by MOPSO algorithm when the weight coefficient of the two objectives set as 0.5.Entities:
Keywords: Ethylene Propylene Diene Monomer; acoustic performances; grey relational analysis; multi-objective particle swarm optimization; polyurethane foam composites
Year: 2018 PMID: 30960714 PMCID: PMC6404009 DOI: 10.3390/polym10070788
Source DB: PubMed Journal: Polymers (Basel) ISSN: 2073-4360 Impact factor: 4.329
Pure polyurethane (PU) foam formulation.
| Raw Materials | Content (g) |
|---|---|
| Polyols (330 N, 3630) | 330 N = 60, 3630 = 40 |
| MDI | 28–32 |
| Catalyst (A1, A33, TEA) | A1 = 0.05, A33 = 1, TEA = 3 |
| Silicone oil | 1.8 |
| Deionized water | 2.5–3.5 |
Design variables and their levels.
| Variables | Parameter Code | Level | ||
|---|---|---|---|---|
| 1 | 2 | 3 | ||
| Content of MDI/g | A | 28 | 30 | 32 |
| Content of EPDM/g | B | 2 | 4 | 6 |
| Hardness of EPDM/HA | C | 65 | 70 | 85 |
| Content of deionized water/g | D | 2.5 | 3 | 3.5 |
Experiment design and experimental results.
| Runs | Variables | Average Sound Absorption Coefficient | Average Transmission Loss/dB | |||
|---|---|---|---|---|---|---|
| A | B | C | D | |||
| 1 | 28 | 2 | 65 | 2.5 | 0.614 | 12.705 |
| 2 | 28 | 4 | 70 | 3 | 0.577 | 14.385 |
| 3 | 28 | 6 | 85 | 3.5 | 0.573 | 16.792 |
| 4 | 30 | 2 | 85 | 3 | 0.511 | 20.887 |
| 5 | 30 | 4 | 65 | 3.5 | 0.574 | 16.298 |
| 6 | 30 | 6 | 70 | 2.5 | 0.580 | 13.991 |
| 7 | 32 | 2 | 70 | 3.5 | 0.521 | 22.272 |
| 8 | 32 | 4 | 85 | 2.5 | 0.557 | 18.445 |
| 9 | 32 | 6 | 65 | 3 | 0.524 | 19.826 |
| 10 | 28 | 4 | 65 | 3 | 0.607 | 10.762 |
| 11 | 28 | 6 | 65 | 2.5 | 0.637 | 9.789 |
| 12 | 30 | 4 | 85 | 3 | 0.543 | 19.906 |
| 13 | 30 | 6 | 70 | 3 | 0.519 | 21.445 |
| 14 | 32 | 6 | 85 | 3 | 0.528 | 20.175 |
| 15 | 32 | 4 | 70 | 3.5 | 0.507 | 24.570 |
Calculation results of normalized sequences, grey relational coefficient and grey relational grade (GRG).
| Runs | Normalized Sequences | Grey Relational Coefficient | GRG | ||
|---|---|---|---|---|---|
| Average Sound Absorption Coefficient | Average Transmission Loss | Average Sound Absorption Coefficient | Average Transmission Loss/dB | ||
| 1 | 1.000 | 0.000 | 1.000 | 0.333 | 0.667 |
| 2 | 0.641 | 0.176 | 0.582 | 0.378 | 0.48 |
| 3 | 0.602 | 0.427 | 0.557 | 0.466 | 0.512 |
| 4 | 0.000 | 0.855 | 0.333 | 0.775 | 0.554 |
| 5 | 0.612 | 0.376 | 0.563 | 0.445 | 0.504 |
| 6 | 0.670 | 0.134 | 0.602 | 0.366 | 0.484 |
| 7 | 0.097 | 1.000 | 0.356 | 1.000 | 0.678 |
| 8 | 0.447 | 0.600 | 0.475 | 0.556 | 0.516 |
| 9 | 0.126 | 0.744 | 0.364 | 0.661 | 0.513 |
Calculation results of average GRG.
| Variables | Average GRG | Range | ||
|---|---|---|---|---|
| Level 1 | Level 2 | Level 3 | ||
| A | 0.553 | 0.514 | 0.569 | 0.055 |
| B | 0.633 | 0.5 | 0.503 | 0.13 |
| C | 0.561 | 0.547 | 0.527 | 0.034 |
| D | 0.556 | 0.516 | 0.565 | 0.049 |
Experimental sample for accuracy evaluation of surrogate models.
| Runs | Variables | Average Sound Absorption Coefficient | Average Transmission Loss/dB | |||
|---|---|---|---|---|---|---|
| A | B | C | D | |||
| 1 | 30 | 2 | 65 | 3 | 0.567 | 15.912 |
| 2 | 30 | 6 | 65 | 3 | 0.551 | 17.914 |
| 3 | 30 | 4 | 70 | 3 | 0.533 | 19.635 |
| 4 | 30 | 4 | 65 | 3 | 0.561 | 16.212 |
| 5 | 32 | 2 | 85 | 3 | 0.481 | 23.801 |
Evaluation coefficients of the surrogate models.
| Objectives | Surrogate Models | DC | RAAE | RMAE |
|---|---|---|---|---|
|
| RS model | 0.9507 | 0.0664 | 0.1402 |
| Kriging model | 0.6440 | 0.1521 | 0.4399 | |
| RBFNN model | 0.8073 | 0.1203 | 0.3115 | |
|
| RS model | 0.9653 | 0.0583 | 0.0968 |
| Kriging model | 0.6793 | 0.1846 | 0.3280 | |
| RBFNN model | 0.9229 | 0.0810 | 0.1695 |
Figure 1Pareto solutions of Response Surface (RS) model.
Figure 2(a) Effect of chemical compositions on sound absorption ability; (b) Effect of functional particle on sound absorption ability; (c) Effect of chemical compositions on sound insulation ability; and (d) Effect of functional particle on sound insulation ability.
Optimization results of simulation and actual experimental.
| Methods | Content of MDI/g | Content of EPDM/g | Hardness of EPDM/HA | Content of Deionized Water/g | Average Sound Absorption Coefficient | Average Transmission Loss/dB | |
|---|---|---|---|---|---|---|---|
| GRA | Experiment | 32 | 2 | 65 | 3.5 | 0.552 | 20.221 |
| Simulation | 32 | 2 | 65 | 3.5 | 0.532 | 21.666 | |
| Error | —— | —— | —— | —— | −0.02 | 1.445 | |
| MOPSO | Experiment | 32 | 5.8 | 65 | 3.4 | 0.519 | 25.764 |
| Simulation | 32 | 5.8 | 65 | 3.4 | 0.512 | 25.85 | |
| Error | —— | —— | —— | —— | −0.007 | 0.086 | |
Figure 3Acoustic performances curve of the PU foam composites (a) Sound absorption coefficient curves; and, (b) Transmission loss curves.