High Performance Plasmonic Nanolasers with External Quantum Efficiency Exceeding 10.

Plasmonic nanolasers break the diffraction limit for an optical oscillator, which brings new capabilities for various applications ranging from on-chip optical interconnector to biomedical sensing and imaging. However, the inevitably accompanied metallic absorption loss could convert the input power to heat rather than radiations, leading to undesired low external quantum efficiency and device degradation. To date, direct characterization of quantum efficiency of plasmonic nanolasers is still a forbidden task due to its near-field surface plasmon emissions, divergent emission profile, and the limited emission power. Here, we develop a method to characterize the external quantum efficiency of plasmonic nanolasers by synergizing experimental measurement and theoretical calculation. With systematical device optimization, we demonstrate high performance plasmonic nanolasers with external quantum efficiency exceeding 10% at room temperature. This work fills in a missing yet essential piece of key metrics of plasmonic nanolasers. The demonstrated high external quantum efficiency of plasmonic nanolasers not only clarifies the long-standing debate, but also endorses the exploration of them in various practical applications such as near-field spectroscopy and sensing, integrated optical interconnects, solid-state lighting, and free-space optical communication.