Antenna-enhanced high harmonic generation in a wide-bandgap semiconductor ZnO.

High harmonic generation (HHG) in solids has great potential for coherent extreme ultraviolet (EUV) sources, all-optical band-structure reconstruction, and electron dynamics metrology. Solid HHG driven by plasmonic near-fields will open a new paradigm, enabling high repetition-rate HHG with a compact laser, HHG manipulation with meta-surfaces, and precise control over carrier trajectory. In this paper, we demonstrate antenna-enhanced HHG in a wide-bandgap semiconductor ZnO. By exploiting gold nano-antennas resonating at the driver wavelength of 2 μm, we successfully trigger HHG at input intensity of ~0.02 TW/cm2 and observe harmonic radiations up to 9th-order. Orders-of-magnitude enhanced conversion efficiency at the hot-spots brings about ten-fold enhancement in the total yield. The spectral selection rule is found to reflect crystal symmetry, suggesting the possibility of nano-scaled EUV sources and band-structure reconstruction.