Literature DB >> 30082905

Quantum spin liquids unveil the genuine Mott state.

A Pustogow1, M Bories2, A Löhle2, R Rösslhuber2, E Zhukova3, B Gorshunov3, S Tomić4, J A Schlueter5,6, R Hübner2,7, T Hiramatsu8, Y Yoshida8,9, G Saito8,10, R Kato11, T-H Lee12, V Dobrosavljević12, S Fratini13, M Dressel2.   

Abstract

The localization of charge carriers by electronic repulsion was suggested by Mott in the 1930s to explain the insulating state observed in supposedly metallic NiO. The Mott metal-insulator transition has been subject of intense investigations ever since1-3-not least for its relation to high-temperature superconductivity4. A detailed comparison to real materials, however, is lacking because the pristine Mott state is commonly obscured by antiferromagnetism and a complicated band structure. Here we study organic quantum spin liquids, prototype realizations of the single-band Hubbard model in the absence of magnetic order. Mapping the Hubbard bands by optical spectroscopy provides an absolute measure of the interaction strength and bandwidth-the crucial parameters that enter calculations. In this way, we advance beyond conventional temperature-pressure plots and quantitatively compose a generic phase diagram for all genuine Mott insulators based on the absolute strength of the electronic correlations. We also identify metallic quantum fluctuations as a precursor of the Mott insulator-metal transition, previously predicted but never observed. Our results suggest that all relevant phenomena in the phase diagram scale with the Coulomb repulsion U, which provides a direct link to unconventional superconductivity in cuprates and other strongly correlated materials.

Year:  2018        PMID: 30082905     DOI: 10.1038/s41563-018-0140-3

Source DB:  PubMed          Journal:  Nat Mater        ISSN: 1476-1122            Impact factor:   43.841


  3 in total

1.  Continuous Mott transition in semiconductor moiré superlattices.

Authors:  Tingxin Li; Shengwei Jiang; Lizhong Li; Yang Zhang; Kaifei Kang; Jiacheng Zhu; Kenji Watanabe; Takashi Taniguchi; Debanjan Chowdhury; Liang Fu; Jie Shan; Kin Fai Mak
Journal:  Nature       Date:  2021-09-15       Impact factor: 69.504

2.  Charge-Ordering and Structural Transition in the New Organic Conductor δ'-(BEDT-TTF)2CF3CF2SO3.

Authors:  Iwona Olejniczak; Bolesław Barszcz; Pascale Auban-Senzier; Harald O Jeschke; Roman Wojciechowski; John A Schlueter
Journal:  J Phys Chem C Nanomater Interfaces       Date:  2022-01-25       Impact factor: 4.126

3.  Rise and fall of Landau's quasiparticles while approaching the Mott transition.

Authors:  Andrej Pustogow; Yohei Saito; Anja Löhle; Miriam Sanz Alonso; Atsushi Kawamoto; Vladimir Dobrosavljević; Martin Dressel; Simone Fratini
Journal:  Nat Commun       Date:  2021-03-10       Impact factor: 14.919

  3 in total

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