A Multifunctional Dye-doped Liquid Crystal Polymer Actuator: Light-Guided Transportation, Turning in Locomotion, and Autonomous Motion.

A strip of a liquid crystal elastomer doped with a near-infrared dye with one side crosslinked monodomain and the other crosslinked polydomain along the thickness behaves like a multifunctional photoactuator without the need for a support. A flat strip with two ends fixed on substrate surface forms a moving bump under laser scanning, which can be used as light-fueled conveyor to transport an object. Cutting off and laser scanning the bump with two free ends makes a soft and flexible millimeter-scale crawler that can not only move straight and climb an inclined surface, but also undergo light-guided turning to right or left as a result of combined out-of-plane and in-plane actuation. Based on the self-shadowing mechanism, with one end of the strip fixed on substrate surface, it can execute a variety of autonomous arm-like movements under constant laser illumination, such as bending-unbending and twisting, depending on the laser incident angles with respect to the strip actuator.