Literature DB >> 29935525

Perspective: How to understand electronic friction.

Wenjie Dou1, Joseph E Subotnik1.   

Abstract

Electronic friction is a correction to the Born-Oppenheimer approximation, whereby nuclei in motion experience a drag in the presence of a manifold of electronic states. The notion of electronic friction has a long history and has been (re-)discovered in the context of a wide variety of different chemical and physical systems including, but not limited to, surface scattering events, surface reactions or chemisorption, electrochemistry, and conduction through molecular-(or nano-) junctions. Over the years, quite a few different forms of electronic friction have been offered in the literature. In this perspective, we briefly review these developments of electronic friction, highlighting the fact that we can now isolate a single, unifying form for (Markovian) electronic friction. We also focus on the role of electron-electron interactions for understanding frictional effects and offer our thoughts on the strengths and weaknesses of using electronic friction to model dynamics in general.

Year:  2018        PMID: 29935525     DOI: 10.1063/1.5035412

Source DB:  PubMed          Journal:  J Chem Phys        ISSN: 0021-9606            Impact factor:   3.488


  5 in total

1.  Determining the Effect of Hot Electron Dissipation on Molecular Scattering Experiments at Metal Surfaces.

Authors:  Connor L Box; Yaolong Zhang; Rongrong Yin; Bin Jiang; Reinhard J Maurer
Journal:  JACS Au       Date:  2020-12-22

Review 2.  Quantitative molecular simulations.

Authors:  Kai Töpfer; Meenu Upadhyay; Markus Meuwly
Journal:  Phys Chem Chem Phys       Date:  2022-06-01       Impact factor: 3.945

3.  Water and carbon make a quantum couple.

Authors: 
Journal:  Nature       Date:  2022-02-02       Impact factor: 49.962

4.  Electronic spin separation induced by nuclear motion near conical intersections.

Authors:  Yanze Wu; Joseph E Subotnik
Journal:  Nat Commun       Date:  2021-01-29       Impact factor: 14.919

5.  Random Force in Molecular Dynamics with Electronic Friction.

Authors:  Nils Hertl; Raidel Martin-Barrios; Oihana Galparsoro; Pascal Larrégaray; Daniel J Auerbach; Dirk Schwarzer; Alec M Wodtke; Alexander Kandratsenka
Journal:  J Phys Chem C Nanomater Interfaces       Date:  2021-06-27       Impact factor: 4.126

  5 in total

北京卡尤迪生物科技股份有限公司 © 2022-2023.