Literature DB >> 29767444

MOF Scaffold for a High-Performance Mixed-Matrix Membrane.

Ke Xie1, Qiang Fu1, Paul A Webley1, Greg G Qiao1.   

Abstract

A novel composite membrane consisting of an interconnected MOF scaffold coated with cross-linked poly(ethylene glycol) (PEG) has been developed. As a result of its unique structure, the membrane shows an exceptional 18-fold permeability enhancement as compared to pristine PEG membranes, without compromising the selectivity. This performance is unattainable with current mixed-matrix membranes (MMMs). Our optimized membrane has a permeability of 2700 Barrer with a CO2 /N2 selectivity of 35, which surpasses the latest Robeson upper bound.
© 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Entities:  

Keywords:  MOF nonwoven cloths; bicontinuous phases; membranes; one-dimensional metal-organic frameworks; polymers

Year:  2018        PMID： 29767444     DOI： 10.1002/anie.201804162

Source DB:  PubMed          Journal:  Angew Chem Int Ed Engl        ISSN： 1433-7851            Impact factor:   15.336


  5 in total

Review 1.  Postsynthetic Modification: An Enabling Technology for the Advancement of Metal-Organic Frameworks.

Authors:  Mark Kalaj; Seth M Cohen
Journal:  ACS Cent Sci       Date:  2020-07-02       Impact factor: 14.553

Review 2.  Performance of Mixed Matrix Membranes Containing Porous Two-Dimensional (2D) and Three-Dimensional (3D) Fillers for CO₂ Separation: A Review.

Authors:  Mahdi Ahmadi; Saravanan Janakiram; Zhongde Dai; Luca Ansaloni; Liyuan Deng
Journal:  Membranes (Basel)       Date:  2018-07-28

3.  A generalizable method for the construction of MOF@polymer functional composites through surface-initiated atom transfer radical polymerization.

Authors:  Sanfeng He; Hongliang Wang; Cuizheng Zhang; Songwei Zhang; Yi Yu; Yongjin Lee; Tao Li
Journal:  Chem Sci       Date:  2018-12-12       Impact factor: 9.825

4.  Ultrapermeable Composite Membranes Enhanced Via Doping with Amorphous MOF Nanosheets.

Authors:  Min Liu; Ke Xie; Mitchell D Nothling; Lianhai Zu; Shenlong Zhao; Dalton J E Harvie; Qiang Fu; Paul A Webley; Greg G Qiao
Journal:  ACS Cent Sci       Date:  2021-03-25       Impact factor: 14.553

5.  Poly(lauryl methacrylate)-Grafted Amino-Functionalized Zirconium-Terephthalate Metal-Organic Framework: Efficient Adsorbent for Extraction of Polycyclic Aromatic Hydrocarbons from Water Samples.

Authors:  Maryam Tabatabaii; Mostafa Khajeh; Ali Reza Oveisi; Mustafa Erkartal; Unal Sen
Journal:  ACS Omega       Date:  2020-05-20
  5 in total

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