Heavy-duty diesel vehicles dominate vehicle emissions in a tunnel study in northern China.

The relative importance of contributions of gasoline vehicles (GVs) and diesel vehicles (DVs), heavy-duty diesel vehicles (HDDVs) and non-HDDVs to on-road vehicle emissions remains unclear. Vehicle emission factors (EFs), including fine particulate matter (PM2.5), NO-NO2-NOx, and carbon monoxide (CO), were measured (August 4-18, 2017) in an urban tunnel in Tianjin, northern China. The average EFs (mg km-1 veh-1) of the fleet were as follows: 9.21 (95% confidence interval: 1.60, 23.07) for PM2.5, 62.08 (21.21, 138.25) for NO, 20.42 (0.79, 45.48) for NO2, 83.72 (26.29, 162.87) for NOx, and 284.54 (18.22, 564.67) for CO. The fleet-average EFs exhibited diurnal variations, due to diurnal variations in the proportion of HDDVs in the fleet, though the hourly proportion of HDDVs never exceeded 10% during the study period. The reconstructed average EFs for on-road vehicle emissions of PM2.5, NO, NO2, and NOx, and CO were approximately 2.2, 1.7, 1.5, 2.0, and 1.6 times as much as those in the tunnel, respectively, due to the higher HDDV fractions in the whole city than those in the tunnel. The EFs of PM2.5, NO, NO2, and NOx, and CO from each HDDV were approximately 75, 81, 24, 65, and 33 times of those from each non-HDDV, respectively. HDDVs were responsible for approximately 81.92%, 83.02%, 59.79%, 79.79%, and 66.77% of the total PM2.5, NO, NO2, and NOx, and CO emissions from on-road vehicles in Tianjin, respectively. DVs, especially HDDVs, are major sources of on-road PM2.5, NO-NO2-NOx, and CO emissions in northern China. The contribution of HDDVs to fleet emissions calculated by the EFs from Chinese 'on-road vehicle emission inventory guidebook' were underestimated, as compared to our results. The EFs from on-road vehicles should be updated due to the rapid progression of vehicle technology combined with emission standards in China. The management and control of HDDV emissions have become urgent to reduction of on-road vehicle emissions.