Literature DB >> 29219594

Phase Competition in the Palmer-Chalker XY Pyrochlore Er_{2}Pt_{2}O_{7}.

A M Hallas1, J Gaudet1, N P Butch2, Guangyong Xu2, M Tachibana3, C R Wiebe1,4,5, G M Luke1,5, B D Gaulin1,5,6.   

Abstract

We report neutron scattering measurements on Er_{2}Pt_{2}O_{7}, a new addition to the XY family of frustrated pyrochlore magnets. Symmetry analysis of our elastic scattering data shows that Er_{2}Pt_{2}O_{7} orders into the k=0, Γ_{7} magnetic structure (the Palmer-Chalker state), at T_{N}=0.38  K. This contrasts with its sister XY pyrochlore antiferromagnets Er_{2}Ti_{2}O_{7} and Er_{2}Ge_{2}O_{7}, both of which order into Γ_{5} magnetic structures at much higher temperatures, T_{N}=1.2 and 1.4 K, respectively. In this temperature range, the magnetic heat capacity of Er_{2}Pt_{2}O_{7} contains a broad anomaly centered at T^{*}=1.5  K. Our inelastic neutron scattering measurements reveal that this broad heat capacity anomaly sets the temperature scale for strong short-range spin fluctuations. Below T_{N}=0.38  K, Er_{2}Pt_{2}O_{7} displays a gapped spin-wave spectrum with an intense, flat band of excitations at lower energy and a weak, diffusive band of excitations at higher energy. The flat band is well described by classical spin-wave calculations, but these calculations also predict sharp dispersive branches at higher energy, a striking discrepancy with the experimental data. This, in concert with the strong suppression of T_{N}, is attributable to enhanced quantum fluctuations due to phase competition between the Γ_{7} and Γ_{5} states that border each other within a classically predicted phase diagram.

Entities:  

Year:  2017        PMID: 29219594     DOI: 10.1103/PhysRevLett.119.187201

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  1 in total

1.  Multiphase magnetism in Yb2Ti2O7.

Authors:  Allen Scheie; Jonas Kindervater; Shu Zhang; Hitesh J Changlani; Gabriele Sala; Georg Ehlers; Andre Heinemann; Gregory S Tucker; Seyed M Koohpayeh; Collin Broholm
Journal:  Proc Natl Acad Sci U S A       Date:  2020-10-23       Impact factor: 11.205

  1 in total

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