| Literature DB >> 28952768 |
Kaiyuan Yao1,2, Aiming Yan3,4, Salman Kahn3, Aslihan Suslu5, Yufeng Liang1, Edward S Barnard1, Sefaattin Tongay5, Alex Zettl3,4,6, Nicholas J Borys1,7, P James Schuck1,8.
Abstract
Optoelectronic excitations in monolayer MoS_{2} manifest from a hierarchy of electrically tunable, Coulombic free-carrier and excitonic many-body phenomena. Investigating the fundamental interactions underpinning these phenomena-critical to both many-body physics exploration and device applications-presents challenges, however, due to a complex balance of competing optoelectronic effects and interdependent properties. Here, optical detection of bound- and free-carrier photoexcitations is used to directly quantify carrier-induced changes of the quasiparticle band gap and exciton binding energies. The results explicitly disentangle the competing effects and highlight longstanding theoretical predictions of large carrier-induced band gap and exciton renormalization in two-dimensional semiconductors.Year: 2017 PMID: 28952768 DOI: 10.1103/PhysRevLett.119.087401
Source DB: PubMed Journal: Phys Rev Lett ISSN: 0031-9007 Impact factor: 9.161