Literature DB >> 28765374

Toward broadband mechanical spectroscopy.

Tina Hecksher1, Darius H Torchinsky2, Christoph Klieber3, Jeremy A Johnson3, Jeppe C Dyre1, Keith A Nelson4.   

Abstract

Diverse material classes exhibit qualitatively similar behavior when made viscous upon cooling toward the glass transition, suggesting a common theoretical basis. We used seven different measurement methods to determine the mechanical relaxation kinetics of a prototype molecular glass former over a temporal range of 13 decades and over a temperature range spanning liquid to glassy states. The data conform to time-temperature superposition for the main (alpha) process and to a scaling relation of schematic mode-coupling theory. The broadband mechanical measurements demonstrated have fundamental and practical applications in polymer science, geophysics, multifunctional materials, and other areas.

Entities:  

Keywords:  broadband mechanical spectroscopy; mode-coupling theory; viscous liquids

Year:  2017        PMID: 28765374      PMCID: PMC5565458          DOI: 10.1073/pnas.1707251114

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  19 in total

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Authors:  N B Olsen; T Christensen; J C Dyre
Journal:  Phys Rev Lett       Date:  2001-02-12       Impact factor: 9.161

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Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1994-06-01

3.  Light scattering study on the glass former o-terphenyl.

Authors:  N Petzold; E A Rössler
Journal:  J Chem Phys       Date:  2010-09-28       Impact factor: 3.488

4.  Dynamical exchanges in facilitated models of supercooled liquids.

Authors:  YounJoon Jung; Juan P Garrahan; David Chandler
Journal:  J Chem Phys       Date:  2005-08-22       Impact factor: 3.488

5.  Solidity of viscous liquids. IV. Density fluctuations.

Authors:  Jeppe C Dyre
Journal:  Phys Rev E Stat Nonlin Soft Matter Phys       Date:  2006-08-04

6.  The influence of shape on the glassy dynamics of hard nonspherical particle fluids. II. Barriers, relaxation, fragility, kinetic vitrification, and universality.

Authors:  Mukta Tripathy; Kenneth S Schweizer
Journal:  J Chem Phys       Date:  2009-06-28       Impact factor: 3.488

7.  A cryostat and temperature control system optimized for measuring relaxations of glass-forming liquids.

Authors:  Brian Igarashi; Tage Christensen; Ebbe H Larsen; Niels Boye Olsen; Ib H Pedersen; Torben Rasmussen; Jeppe C Dyre
Journal:  Rev Sci Instrum       Date:  2008-04       Impact factor: 1.523

8.  Surface generation and detection of phonons by picosecond light pulses.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1986-09-15

9.  Testing mode-coupling predictions for alpha and beta relaxation in Ca0.4K0.6(NO3)1.4 near the liquid-glass transition by light scattering.

Authors: 
Journal:  Phys Rev A       Date:  1992-03-15       Impact factor: 3.140

10.  Light-scattering investigation of alpha and beta relaxation near the liquid-glass transition of the molecular glass Salol.

Authors: 
Journal:  Phys Rev A       Date:  1992-09-15       Impact factor: 3.140

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  1 in total

1.  Evidence of a one-dimensional thermodynamic phase diagram for simple glass-formers.

Authors:  H W Hansen; A Sanz; K Adrjanowicz; B Frick; K Niss
Journal:  Nat Commun       Date:  2018-02-06       Impact factor: 14.919

  1 in total

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