Literature DB >> 28644632

Mott Transition in the A15 Phase of Cs_{3}C_{60}: Absence of a Pseudogap and Charge Order.

H Alloul1, P Wzietek1, T Mito1, D Pontiroli2, M Aramini2,3, M Riccò2, J P Itie4, E Elkaim4.   

Abstract

We present a detailed NMR study of the insulator-to-metal transition induced by an applied pressure p in the A15 phase of Cs_{3}C_{60}. We evidence that the insulating antiferromagnetic (AFM) and superconducting (SC) phases coexist only in a narrow p range. At fixed p, in the metallic state above the SC transition T_{c}, the ^{133}Cs and ^{13}C NMR spin-lattice relaxation data are seemingly governed by a pseudogaplike feature. We prove that this feature, also seen in the ^{133}Cs NMR shift data, is rather a signature of the Mott transition which broadens and smears out progressively for increasing (p,T). The analysis of the variation of the quadrupole splitting ν_{Q} of the ^{133}Cs NMR spectrum precludes any cell symmetry change at the Mott transition and only monitors a weak variation of the lattice parameter. These results open an opportunity to consider theoretically the Mott transition in a multiorbital three-dimensional system well beyond its critical point.

Entities:  

Year:  2017        PMID: 28644632     DOI: 10.1103/PhysRevLett.118.237601

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  1 in total

1.  Synthesis and structural analysis of nonstoichiometric ternary fulleride K 1.5 Ba 0.25 CsC 60.

Authors:  Havva Esma Okur Kutay
Journal:  Turk J Chem       Date:  2020-12-16       Impact factor: 1.239

  1 in total

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