| Literature DB >> 28462970 |
Holger Merlitz1, Chenxu Wu, Jens-Uwe Sommer.
Abstract
We present a setup in which passive colloids inside a solvent are moved to the boundaries of the container. The directional transport is facilitated by self-propelling microparticles ("walkers") with an activity gradient, which reduces their propulsion in the vicinity of bounding walls. An attractive interaction leads to the adsorption of walkers onto the colloid-surfaces in regions of low walker activity. It is shown that the activity gradient generates a free energy gradient which in turn acts as a driving force on the passive colloids. We carry out molecular dynamics simulations and present approaches to a theoretical description of the involved processes. Although the simulation data are not reproduced on a fully quantitative level, their qualitative features are covered by the model. The effect described here may be applied to facilitate a directional transport of drugs or to eliminate pollutants.Year: 2017 PMID: 28462970 DOI: 10.1039/c7sm00613f
Source DB: PubMed Journal: Soft Matter ISSN: 1744-683X Impact factor: 3.679