Literature DB >> 28169520

Hydrogen Gas Recycling for Energy Efficient Ammonia Recovery in Electrochemical Systems.

Philipp Kuntke1, Mariana Rodríguez Arredondo1,2, Laksminarastri Widyakristi1, Annemiek Ter Heijne2, Tom H J A Sleutels1, Hubertus V M Hamelers1, Cees J N Buisman1,2.   

Abstract

Recycling of hydrogen gas (H2) produced at the cathode to the anode in an electrochemical system allows for energy efficient TAN (Total Ammonia Nitrogen) recovery. Using a H2 recycling electrochemical system (HRES) we achieved high TAN transport rates at low energy input. At a current density of 20 A m-2, TAN removal rate from the influent was 151 gN m-2 d-1 at an energy demand of 26.1 kJ gN-1. The maximum TAN transport rate of 335 gN m-2 d-1 was achieved at a current density of 50 A m-2 and an energy demand of 56.3 kJ gN-1. High TAN removal efficiency (73-82%) and recovery (60-73%) were reached in all experiments. Therefore, our HRES is a promising alternative for electrochemical and bioelectrochemical TAN recovery. Advantages are the lower energy input and lower risk of chloride oxidation compared to electrochemical technologies and high rates and independence of organic matter compared to bioelectrochemical systems.

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Year:  2017        PMID: 28169520     DOI: 10.1021/acs.est.6b06097

Source DB:  PubMed          Journal:  Environ Sci Technol        ISSN: 0013-936X            Impact factor:   9.028


  7 in total

1.  Energy-Efficient Ammonia Recovery in an Up-Scaled Hydrogen Gas Recycling Electrochemical System.

Authors:  Philipp Kuntke; Mariana Rodrigues; Tom Sleutels; Michel Saakes; Hubertus V M Hamelers; Cees J N Buisman
Journal:  ACS Sustain Chem Eng       Date:  2018-05-08       Impact factor: 8.198

Review 2.  (Bio)electrochemical ammonia recovery: progress and perspectives.

Authors:  P Kuntke; T H J A Sleutels; M Rodríguez Arredondo; S Georg; S G Barbosa; A Ter Heijne; Hubertus V M Hamelers; C J N Buisman
Journal:  Appl Microbiol Biotechnol       Date:  2018-03-09       Impact factor: 4.813

Review 3.  Urine in Bioelectrochemical Systems: An Overall Review.

Authors:  Carlo Santoro; Maria Jose Salar Garcia; Xavier Alexis Walter; Jiseon You; Pavlina Theodosiou; Iwona Gajda; Oluwatosin Obata; Jonathan Winfield; John Greenman; Ioannis Ieropoulos
Journal:  ChemElectroChem       Date:  2020-03-06       Impact factor: 4.590

4.  Minimal Bipolar Membrane Cell Configuration for Scaling Up Ammonium Recovery.

Authors:  Mariana Rodrigues; Thiago T de Mattos; Tom Sleutels; Annemiek Ter Heijne; Hubertus V M Hamelers; Cees J N Buisman; Philipp Kuntke
Journal:  ACS Sustain Chem Eng       Date:  2020-11-18       Impact factor: 8.198

5.  Effects of Current on the Membrane and Boundary Layer Selectivity in Electrochemical Systems Designed for Nutrient Recovery.

Authors:  Mariana Rodrigues; Tom Sleutels; Philipp Kuntke; Cees J N Buisman; Hubertus V M Hamelers
Journal:  ACS Sustain Chem Eng       Date:  2022-07-15       Impact factor: 9.224

6.  Direct Air Capture Using Electrochemically Regenerated Anion Exchange Resins.

Authors:  Qingdian Shu; Marina Haug; Michele Tedesco; Philipp Kuntke; Hubertus V M Hamelers
Journal:  Environ Sci Technol       Date:  2022-08-04       Impact factor: 11.357

Review 7.  The Application of Cation Exchange Membranes in Electrochemical Systems for Ammonia Recovery from Wastewater.

Authors:  Kai Yang; Mohan Qin
Journal:  Membranes (Basel)       Date:  2021-06-30
  7 in total

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