Literature DB >> 28128620

Doping Evolution of Magnetic Order and Magnetic Excitations in (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7}.

Xingye Lu1, D E McNally1, M Moretti Sala2, J Terzic3,4, M H Upton5, D Casa5, G Ingold1,6, G Cao3,4, T Schmitt1.   

Abstract

We use resonant elastic and inelastic x-ray scattering at the Ir-L_{3} edge to study the doping-dependent magnetic order, magnetic excitations, and spin-orbit excitons in the electron-doped bilayer iridate (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7} (0≤x≤0.065). With increasing doping x, the three-dimensional long range antiferromagnetic order is gradually suppressed and evolves into a three-dimensional short range order across the insulator-to-metal transition from x=0 to 0.05, followed by a transition to two-dimensional short range order between x=0.05 and 0.065. Because of the interactions between the J_{eff}=1/2 pseudospins and the emergent itinerant electrons, magnetic excitations undergo damping, anisotropic softening, and gap collapse, accompanied by weakly doping-dependent spin-orbit excitons. Therefore, we conclude that electron doping suppresses the magnetic anisotropy and interlayer couplings and drives (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7} into a correlated metallic state with two-dimensional short range antiferromagnetic order. Strong antiferromagnetic fluctuations of the J_{eff}=1/2 moments persist deep in this correlated metallic state, with the magnon gap strongly suppressed.

Entities:  

Year:  2017        PMID: 28128620     DOI: 10.1103/PhysRevLett.118.027202

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  4 in total

1.  Laser-induced transient magnons in Sr3Ir2O7 throughout the Brillouin zone.

Authors:  Daniel G Mazzone; Derek Meyers; Yue Cao; James G Vale; Cameron D Dashwood; Youguo Shi; Andrew J A James; Neil J Robinson; Jiaqi Lin; Vivek Thampy; Yoshikazu Tanaka; Allan S Johnson; Hu Miao; Ruitang Wang; Tadesse A Assefa; Jungho Kim; Diego Casa; Roman Mankowsky; Diling Zhu; Roberto Alonso-Mori; Sanghoon Song; Hasan Yavas; Tetsuo Katayama; Makina Yabashi; Yuya Kubota; Shigeki Owada; Jian Liu; Junji Yang; Robert M Konik; Ian K Robinson; John P Hill; Desmond F McMorrow; Michael Först; Simon Wall; Xuerong Liu; Mark P M Dean
Journal:  Proc Natl Acad Sci U S A       Date:  2021-06-01       Impact factor: 11.205

2.  Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator.

Authors:  He Zhao; Zach Porter; Xiang Chen; Stephen D Wilson; Ziqiang Wang; Ilija Zeljkovic
Journal:  Sci Adv       Date:  2021-11-10       Impact factor: 14.136

3.  Antiferromagnetic excitonic insulator state in Sr3Ir2O7.

Authors:  D G Mazzone; Y Shen; H Suwa; G Fabbris; J Yang; S-S Zhang; H Miao; J Sears; Ke Jia; Y G Shi; M H Upton; D M Casa; X Liu; Jian Liu; C D Batista; M P M Dean
Journal:  Nat Commun       Date:  2022-02-17       Impact factor: 14.919

4.  Quantum Spin-1/2 Dimers in a Low-Dimensional Tetrabromocuprate Magnet.

Authors:  Gavin Sampson; Nicholas C Bristowe; Sam T Carr; Asad Saib; Gavin B G Stenning; Ewan R Clark; Paul J Saines
Journal:  Chemistry       Date:  2022-04-27       Impact factor: 5.020

  4 in total

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