Literature DB >> 28055106

Imidazoquinoxaline derivative EAPB0503: A promising drug targeting mutant nucleophosmin 1 in acute myeloid leukemia.

Ali I Nabbouh1,2, Rita S Hleihel1,3, Jessica L Saliba4, Martin M Karam1,5, Maguy H Hamie1,5, Hsin-Chieh J M Wu6, Caroline P Berthier6, Nadim M Tawil7, Pierre-Antoine A Bonnet2, Carine Deleuze-Masquefa2, Hiba A El Hajj1,5.   

Abstract

BACKGROUND: Nucleophosmin 1 (NPM1) is a nucleocytoplasmic shuttling protein mainly localized in the nucleolus. NPM1 is frequently mutated in acute myeloid leukemia (AML). NPM1c oligomerizes with wild-type nucleophosmin 1 (wt-NPM1), and this leads to its continuous cytoplasmic delocalization and contributes to leukemogenesis. Recent studies have shown that Cytoplasmic NPM1 (NPM1c) degradation leads to growth arrest and apoptosis of NPM1c AML cells and corrects wt-NPM1 normal nucleolar localization.
METHODS: AML cells expressing wt-NPM1 or NPM1c or transfected with wt-NPM1 or NPM1c as well as wt-NPM1 and NPM1c AML xenograft mice were used. Cell growth was assessed with trypan blue or a CellTiter 96 proliferation kit. The cell cycle was studied with a propidium iodide (PI) assay. Caspase-mediated intrinsic apoptosis was assessed with annexin V/PI, the mitochondrial membrane potential, and poly(adenosine diphosphate ribose) polymerase cleavage. The expression of NPM1, p53, phosphorylated p53, and p21 was analyzed via immunoblotting. Localization was performed with confocal microscopy. The leukemia burden was evaluated by flow cytometry with an anti-human CD45 antibody.
RESULTS: The imidazoquinoxaline 1-(3-methoxyphenyl)-N-methylimidazo[1,2-a]quinoxalin-4-amine (EAPB0503) induced selective proteasome-mediated degradation of NPM1c, restored wt-NPM1 nucleolar localization in NPM1c AML cells, and thus yielded selective growth arrest and apoptosis. Introducing NPM1c to cells normally harboring wt-NPM1 sensitized them to EAPB0503 and led to their growth arrest. Moreover, EAPB0503 selectively reduced the leukemia burden in NPM1c AML xenograft mice.
CONCLUSIONS: These findings further reinforce the idea of targeting the NPM1c oncoprotein to eradicate leukemic cells and warrant a broader preclinical evaluation and then a clinical evaluation of this promising drug. Cancer 2017;123:1662-1673.
© 2017 American Cancer Society. © 2017 American Cancer Society.

Entities:  

Keywords:  1-(3-methoxyphenyl)-N-methylimidazo[1,2-a]quinoxalin-4-amine (EAPB0503); acute myeloid leukemia; apoptosis; nucleophosmin 1; xenograft mice

Mesh:

Substances:

Year:  2017        PMID: 28055106     DOI: 10.1002/cncr.30515

Source DB:  PubMed          Journal:  Cancer        ISSN: 0008-543X            Impact factor:   6.860


  11 in total

1.  Imiquimod inhibits growth and induces differentiation of myeloid leukemia cell lines.

Authors:  Eva Villamón; Javier González-Fernández; Esperanza Such; José Vicente Cervera; Daniel Gozalbo; M Luisa Gil
Journal:  Cancer Cell Int       Date:  2018-01-30       Impact factor: 5.722

Review 2.  Proteolysis targeting chimeras (PROTACs) are emerging therapeutics for hematologic malignancies.

Authors:  Yonghan He; Sajid Khan; Zhiguang Huo; Dongwen Lv; Xuan Zhang; Xingui Liu; Yaxia Yuan; Robert Hromas; Mingjiang Xu; Guangrong Zheng; Daohong Zhou
Journal:  J Hematol Oncol       Date:  2020-07-27       Impact factor: 17.388

3.  Differential expression of NPM, GSTA3, and GNMT in mouse liver following long-term in vivo irradiation by means of uranium tailings.

Authors:  Lan Yi; Hongxiang Mu; Nan Hu; Jing Sun; Jie Yin; Keren Dai; Dingxin Long; Dexin Ding
Journal:  Biosci Rep       Date:  2018-10-17       Impact factor: 3.840

4.  EAPB0503: An Imiquimod analog with potent in vitro activity against cutaneous leishmaniasis caused by Leishmania major and Leishmania tropica.

Authors:  Rana El Hajj; Hanady Bou Youness; Laurence Lachaud; Patrick Bastien; Carine Masquefa; Pierre-Antoine Bonnet; Hiba El Hajj; Ibrahim Khalifeh
Journal:  PLoS Negl Trop Dis       Date:  2018-11-21

Review 5.  A Critical Review of Animal Models Used in Acute Myeloid Leukemia Pathophysiology.

Authors:  Hala Skayneh; Batoul Jishi; Rita Hleihel; Maguy Hamieh; Nadine Darwiche; Ali Bazarbachi; Marwan El Sabban; Hiba El Hajj
Journal:  Genes (Basel)       Date:  2019-08-13       Impact factor: 4.096

6.  EAPB0503, an Imidazoquinoxaline Derivative Modulates SENP3/ARF Mediated SUMOylation, and Induces NPM1c Degradation in NPM1 Mutant AML.

Authors:  Hala Skayneh; Batoul Jishi; Rita Hleihel; Maguy Hamie; Rana El Hajj; Carine Deleuze-Masquefa; Pierre-Antoine Bonnet; Marwan El Sabban; Hiba El Hajj
Journal:  Int J Mol Sci       Date:  2022-03-22       Impact factor: 5.923

Review 7.  Nucleophosmin 1 Mutations in Acute Myeloid Leukemia.

Authors:  Jabra Zarka; Nicholas J Short; Rashmi Kanagal-Shamanna; Ghayas C Issa
Journal:  Genes (Basel)       Date:  2020-06-12       Impact factor: 4.096

Review 8.  The nucleolus, an ally, and an enemy of cancer cells.

Authors:  Dariusz Stępiński
Journal:  Histochem Cell Biol       Date:  2018-08-13       Impact factor: 4.304

9.  A novel leukemic route of mutant NPM1 through nuclear import of the overexpressed long noncoding RNA LONA.

Authors:  Morgane Gourvest; Etienne De Clara; Hsin-Chieh Wu; Christian Touriol; Fabienne Meggetto; Hugues De Thé; Stéphane Pyronnet; Pierre Brousset; Marina Bousquet
Journal:  Leukemia       Date:  2021-06-15       Impact factor: 11.528

10.  A Pin1/PML/P53 axis activated by retinoic acid in NPM-1c acute myeloid leukemia.

Authors:  Rita Hleihel; Hiba El Hajj; Hsin-Chieh Wu; Caroline Berthier; Hong-Hu Zhu; Radwan Massoud; Zaher Chakhachiro; Marwan El Sabban; Hugues De The; Ali Bazarbachi
Journal:  Haematologica       Date:  2021-12-01       Impact factor: 9.941

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