Literature DB >> 27739762

Point-to-set lengths, local structure, and glassiness.

Sho Yaida1, Ludovic Berthier2, Patrick Charbonneau3, Gilles Tarjus4.   

Abstract

The growing sluggishness of glass-forming liquids is thought to be accompanied by growing structural order. The nature of such order, however, remains hotly debated. A decade ago, point-to-set (PTS) correlation lengths were proposed as measures of amorphous order in glass formers, but recent results raise doubts as to their generality. Here, we extend the definition of PTS correlations to agnostically capture any type of growing order in liquids, be it local or amorphous. This advance enables the formulation of a clear distinction between slowing down due to conventional critical ordering and that due to glassiness, and provides a unified framework to assess the relative importance of specific local order and generic amorphous order in glass formation.

Year:  2016        PMID: 27739762     DOI: 10.1103/PhysRevE.94.032605

Source DB:  PubMed          Journal:  Phys Rev E        ISSN: 2470-0045            Impact factor:   2.529


  4 in total

1.  Glass transitions may be similar in two and three dimensions, after all.

Authors:  Gilles Tarjus
Journal:  Proc Natl Acad Sci U S A       Date:  2017-02-27       Impact factor: 11.205

2.  Real space renormalization group theory of disordered models of glasses.

Authors:  Maria Chiara Angelini; Giulio Biroli
Journal:  Proc Natl Acad Sci U S A       Date:  2017-02-21       Impact factor: 11.205

3.  Measurements of growing surface tension of amorphous-amorphous interfaces on approaching the colloidal glass transition.

Authors:  Divya Ganapathi; K Hima Nagamanasa; A K Sood; Rajesh Ganapathy
Journal:  Nat Commun       Date:  2018-01-26       Impact factor: 14.919

4.  Revisiting the concept of activation in supercooled liquids.

Authors:  Marco Baity-Jesi; Giulio Biroli; David R Reichman
Journal:  Eur Phys J E Soft Matter       Date:  2021-06-14       Impact factor: 1.890

  4 in total

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