Literature DB >> 27682846

Calculated conjugated payload from immunoassay and LC-MS intact protein analysis measurements of antibody-drug conjugate.

Brian Rago1, Tracey Clark1, Lindsay King1, Jenny Zhang2, L Nathan Tumey3, Fengping Li1, Frank Barletta1, Cong Wei1, Mauricio Leal1, Steve Hansel1, Xiaogang Han1,4.   

Abstract

AIM: Complex nature of bioconjugates require multiple bioanalytical approaches to support PK and absorption, distribution, metabolism and excretion characterization. For antibody-drug conjugate (ADC) bioanalysis both LC-MS and ligand-binding assays (LBAs) are employed.
RESULTS: A method consisting of immunocapture extraction of ADC from biomatrices followed by LC-MS analysis of light and heavy chain is described. Drug antibody ratio (DAR) profiles of ADC Tras-mcVC-PF06380101 dosed at 0.3, 1 and 3 mg/kg in Sprague Dawley rats were obtained. Combined with total antibody (monoclonal antibody) measurement by LBA, conjugated payload concentration was calculated.
CONCLUSION: PK profiles from LBA, ADC and calculated conjugated payload (DAR × monoclonal antibody) were in good agreement. We present a new tool for PK assessment of ADCs while also exploring ADC metabolism and DAR sensitivity of LBA ADC assay.

Entities:  

Keywords:  LC–MS; PKs; antibody-drug conjugate; ligand-binding assay; metabolism

Mesh:

Substances:

Year:  2016        PMID: 27682846     DOI: 10.4155/bio-2016-0160

Source DB:  PubMed          Journal:  Bioanalysis        ISSN: 1757-6180            Impact factor:   2.681


  3 in total

1.  Site Selection: a Case Study in the Identification of Optimal Cysteine Engineered Antibody Drug Conjugates.

Authors:  L Nathan Tumey; Fengping Li; Brian Rago; Xiaogang Han; Frank Loganzo; Sylvia Musto; Edmund I Graziani; Sujiet Puthenveetil; Jeffrey Casavant; Kimberly Marquette; Tracey Clark; Jack Bikker; Eric M Bennett; Frank Barletta; Nicole Piche-Nicholas; Amy Tam; Christopher J O'Donnell; Hans Peter Gerber; Lioudmila Tchistiakova
Journal:  AAPS J       Date:  2017-04-24       Impact factor: 4.009

Review 2.  Challenges and new frontiers in analytical characterization of antibody-drug conjugates.

Authors:  Anil Wagh; Hangtian Song; Ming Zeng; Li Tao; Tapan K Das
Journal:  MAbs       Date:  2018-01-05       Impact factor: 5.857

Review 3.  Current LC-MS-based strategies for characterization and quantification of antibody-drug conjugates.

Authors:  Xiaoyu Zhu; Shihan Huo; Chao Xue; Bo An; Jun Qu
Journal:  J Pharm Anal       Date:  2020-05-23
  3 in total

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