Literature DB >> 27636488

Persistent Paramagnons Deep in the Metallic Phase of Sr_{2-x}La_{x}IrO_{4}.

H Gretarsson1, N H Sung1, J Porras1, J Bertinshaw1, C Dietl1, Jan A N Bruin1, A F Bangura1, Y K Kim2,3,4, R Dinnebier1, Jungho Kim5, A Al-Zein6, M Moretti Sala6, M Krisch6, M Le Tacon1,7, B Keimer1, B J Kim1.   

Abstract

We have studied the magnetic excitations of electron-doped Sr_{2-x}La_{x}IrO_{4} (0≤x≤0.10) using resonant inelastic x-ray scattering at the Ir L_{3} edge. The long-range magnetic order is rapidly lost with increasing x, but two-dimensional short-range order (SRO) and dispersive magnon excitations with nearly undiminished spectral weight persist well into the metallic part of the phase diagram. The magnons in the SRO phase are heavily damped and exhibit anisotropic softening. Their dispersions are well described by a pseudospin-1/2 Heisenberg model with exchange interactions whose spatial range increases with doping. We also find a doping-independent high-energy magnetic continuum, which is not described by this model. The spin-orbit excitons arising from the pseudospin-3/2 manifold of the Ir ions broaden substantially in the SRO phase, but remain largely separated from the low-energy magnons. Pseudospin-1/2 models are therefore a good starting point for the theoretical description of the low-energy magnetic dynamics of doped iridates.

Year:  2016        PMID: 27636488     DOI: 10.1103/PhysRevLett.117.107001

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  2 in total

1.  Unidirectional spin density wave state in metallic (Sr1-xLa x )2IrO4.

Authors:  Xiang Chen; Julian L Schmehr; Zahirul Islam; Zach Porter; Eli Zoghlin; Kenneth Finkelstein; Jacob P C Ruff; Stephen D Wilson
Journal:  Nat Commun       Date:  2018-01-09       Impact factor: 14.919

2.  IRIXS: a resonant inelastic X-ray scattering instrument dedicated to X-rays in the intermediate energy range.

Authors:  Hlynur Gretarsson; Didem Ketenoglu; Manuel Harder; Simon Mayer; Frank Uwe Dill; Manfred Spiwek; Horst Schulte-Schrepping; Markus Tischer; Hans Christian Wille; Bernhard Keimer; Hasan Yavaş
Journal:  J Synchrotron Radiat       Date:  2020-02-26       Impact factor: 2.616

  2 in total

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