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Literature DB >> 27622869

Defect Graphene as a Trifunctional Catalyst for Electrochemical Reactions.

Yi Jia^1,2, Longzhou Zhang^1,2, Aijun Du³, Guoping Gao³, Jun Chen⁴, Xuecheng Yan^1,2, Christopher L Brown^2,5, Xiangdong Yao^1,2.

Abstract

Defects derived by the removal of heteroatoms from graphene are demonstrated, both experimentally and theoretically, to be effective for all three basic electrochemical reactions, e.g., oxygen reduction (ORR), oxygen evolution (OER), and hydrogen evolution (HER). Density function theory calculations further reveal that the different types of defects are essential for the individual electrocatalytic activity for ORR, OER, and HER, respectively.

Entities: Chemical

Keywords: defects; electrocatalysts; graphene; hydrogen evolution; oxygen reduction, oxygen evolution

Year: 2016 PMID： 27622869 DOI： 10.1002/adma.201602912

Source DB: PubMed Journal: Adv Mater ISSN： 0935-9648 Impact factor: 30.849

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Cited

29 in total

Review 1. Electrosynthesis of H₂O₂ through a two-electron oxygen reduction reaction by carbon based catalysts: From mechanism, catalyst design to electrode fabrication.

Authors: Jingkun An; Yujie Feng; Qian Zhao; Xin Wang; Jia Liu; Nan Li
Journal: Environ Sci Ecotechnol Date: 2022-03-30

2. Hydrothermal and plasma nitrided electrospun carbon nanofibers for amperometric sensing of hydrogen peroxide.

Authors: Yuan-Ping Lyu; Yi-Shan Wu; Tzu-Pei Wang; Chien-Liang Lee; Meng-Yin Chung; Chieh-Tsung Lo
Journal: Mikrochim Acta Date: 2018-07-10 Impact factor: 5.833

3. Twin boundary defect engineering improves lithium-ion diffusion for fast-charging spinel cathode materials.

Authors: Rui Wang; Xin Chen; Zhongyuan Huang; Jinlong Yang; Fusheng Liu; Mihai Chu; Tongchao Liu; Chaoqi Wang; Weiming Zhu; Shuankui Li; Shunning Li; Jiaxin Zheng; Jie Chen; Lunhua He; Lei Jin; Feng Pan; Yinguo Xiao
Journal: Nat Commun Date: 2021-05-25 Impact factor: 14.919

Review 4. Atomically Dispersed Reactive Centers for Electrocatalytic CO₂ Reduction and Water Splitting.

Authors: Huabin Zhang; Weiren Cheng; Deyan Luan; Xiong Wen David Lou
Journal: Angew Chem Int Ed Engl Date: 2021-02-24 Impact factor: 15.336

5. Exploitation of the Large-Area Basal Plane of MoS₂ and Preparation of Bifunctional Catalysts through On-Surface Self-Assembly.

Authors: Yinghe Zhao; Qiang Li; Li Shi; Jinlan Wang
Journal: Adv Sci (Weinh) Date: 2017-09-23 Impact factor: 16.806

10. The Activity Improvement of the TM₃(hexaiminotriphenylene)₂ Monolayer for Oxygen Reduction Electrocatalysis: A Density Functional Theory Study.

Authors: Beibei Xiao; Hui Zhu; HouYi Liu; XiaoBao Jiang; Qing Jiang
Journal: Front Chem Date: 2018-09-12 Impact factor: 5.221

Defect Graphene as a Trifunctional Catalyst for Electrochemical Reactions.

Review 1. Electrosynthesis of H₂O₂ through a two-electron oxygen reduction reaction by carbon based catalysts: From mechanism, catalyst design to electrode fabrication.

2. Hydrothermal and plasma nitrided electrospun carbon nanofibers for amperometric sensing of hydrogen peroxide.

3. Twin boundary defect engineering improves lithium-ion diffusion for fast-charging spinel cathode materials.

Review 4. Atomically Dispersed Reactive Centers for Electrocatalytic CO₂ Reduction and Water Splitting.

5. Exploitation of the Large-Area Basal Plane of MoS₂ and Preparation of Bifunctional Catalysts through On-Surface Self-Assembly.

Review 6. Recent Progress on Layered Double Hydroxides and Their Derivatives for Electrocatalytic Water Splitting.

7. Induced Ferromagnetic Order of Graphdiyne Semiconductors by Introducing a Heteroatom.

Review 8. Defect Engineering on Carbon-Based Catalysts for Electrocatalytic CO₂ Reduction.

Review 9. Advanced Architectures and Relatives of Air Electrodes in Zn-Air Batteries.

10. The Activity Improvement of the TM₃(hexaiminotriphenylene)₂ Monolayer for Oxygen Reduction Electrocatalysis: A Density Functional Theory Study.

Defect Graphene as a Trifunctional Catalyst for Electrochemical Reactions.

Review 1. Electrosynthesis of H2O2 through a two-electron oxygen reduction reaction by carbon based catalysts: From mechanism, catalyst design to electrode fabrication.

2. Hydrothermal and plasma nitrided electrospun carbon nanofibers for amperometric sensing of hydrogen peroxide.

3. Twin boundary defect engineering improves lithium-ion diffusion for fast-charging spinel cathode materials.

Review 4. Atomically Dispersed Reactive Centers for Electrocatalytic CO2 Reduction and Water Splitting.

5. Exploitation of the Large-Area Basal Plane of MoS2 and Preparation of Bifunctional Catalysts through On-Surface Self-Assembly.

Review 6. Recent Progress on Layered Double Hydroxides and Their Derivatives for Electrocatalytic Water Splitting.

7. Induced Ferromagnetic Order of Graphdiyne Semiconductors by Introducing a Heteroatom.

Review 8. Defect Engineering on Carbon-Based Catalysts for Electrocatalytic CO2 Reduction.

Review 9. Advanced Architectures and Relatives of Air Electrodes in Zn-Air Batteries.

10. The Activity Improvement of the TM3(hexaiminotriphenylene)2 Monolayer for Oxygen Reduction Electrocatalysis: A Density Functional Theory Study.

Review 1. Electrosynthesis of H₂O₂ through a two-electron oxygen reduction reaction by carbon based catalysts: From mechanism, catalyst design to electrode fabrication.

Review 4. Atomically Dispersed Reactive Centers for Electrocatalytic CO₂ Reduction and Water Splitting.

5. Exploitation of the Large-Area Basal Plane of MoS₂ and Preparation of Bifunctional Catalysts through On-Surface Self-Assembly.

Review 8. Defect Engineering on Carbon-Based Catalysts for Electrocatalytic CO₂ Reduction.

10. The Activity Improvement of the TM₃(hexaiminotriphenylene)₂ Monolayer for Oxygen Reduction Electrocatalysis: A Density Functional Theory Study.