We demonstrate the generation of far-field propagating optical beams with a desired orbital angular momentum by using a smooth optical-mode transformation between a plasmonic vortex and free-space Laguerre-Gaussian modes. This is obtained by means of an adiabatically tapered gold tip surrounded by a spiral slit. The proposed physical model, backed up by the numerical study, brings about an optimized structure that is fabricated by using a highly reproducible secondary electron lithography technique. Optical measurements of the structure excellently agree with the theoretically predicted far-field distributions. This architecture provides a unique platform for a localized excitation of plasmonic vortices followed by its beaming.
We demonstrate the generation of far-field propagating optical beams with a desired orbital angular momentum by using a smooth optical-mode transformation between a plasmonic vortex and free-space Laguerre-Gaussian modes. This is obtained by means of an adiabatically tapered gold tip surrounded by a spiral slit. The proposed physical model, backed up by the numerical study, brings about an optimized structure that is fabricated by using a highly reproducible secondary electron lithography technique. Optical measurements of the structure excellently agree with the theoretically predicted far-field distributions. This architecture provides a unique platform for a localized excitation of plasmonic vortices followed by its beaming.
Structured
light beams have been the subject of an intense work in the last years[1,2] due to the numerous potential applications that they may offer in
several disparate technological and research fields, ranging from
super-resolution imaging[3] to optical tweezing[4] and nanomanipulation[5] and telecommunications.[6]The possibility
of producing and analyzing singular optical beams at the micro- and
the nanoscale led to focus on the interaction of light with metallic
nanostructures, resulting in surface plasmon polaritons (SPPs) carrying
angular momentum (AM).[7−13] We will refer to these waves as plasmonic vortices (PVs). Such modes
are generally surface confined helical electromagnetic distributions
with a field singularity. The strength of the singularity, termed
the topological charge of a vortex, is defined by the phase ramp acquired
in one round trip about the singularity center. This charge is proportional
to the AM carried by the field.[10]PVs can be generated by coupling AM-carrying beams to the plasmonic
modes of metallic films using particular chiral grating couplers,
which have been sometimes called plasmonic vortex lenses (PVLs).[10] Several examples of these couplers have been
presented so far.[8−18] A feature common to most of them is the Archimede’s spiral-shaped
grooves or slits milled in a noble metal film.As has been pointed
out in several papers, PVLs can be used not only to couple light to
plasmonic vortices but also to produce strongly localized sources
of light carrying nonzero angular momentum.[9,15,16,19,20] In this case, incident circularly polarized light
interacting with the plasmonic lens excites PV, which is finally scattered
into a free space by a proper decoupling structure.One of the
most studied architectures for this aim consists of a PVL with a hole
at its center.[9,16,20] The drawback of this scheme is a low efficiency and poor directionality
of the far-field beaming due to a small hole size. Moreover, it unavoidably
transmits part of the light directly impinging onto the hole, which
has not been phase-structured by the PVL. More-complex structures,
composed of suspended gold membranes patterned on both sides or multilayer
metal–insulator–metal waveguides, were proposed to address
those issues.[16,20−22] However, besides
an increase in the fabrication complexity, the highly desirable properties
of transmitting a well-defined phase-structured beam with high efficiency
and good directionality have been not fully achieved at the same time.Here, we theoretically and experimentally demonstrate a different
approach to the efficient PV coupling to the free space, by means
of a single-layer PVL structure with a smoothed-cone tip at its center
(Figure a). We show
that, by properly shaping the tip geometry, the PV excited by the
spiral structure can be adiabatically coupled to the far-field mode,
carrying well-defined AM. A crucial role is played by the strong smoothness
of the tip basis. As we shall demonstrate, by simply increasing the
curvature radius at the basis of a conical structure, a totally different
optical behavior can be achieved, enabling a smooth propagation of
the PVs along the tip with a gradual matching to a free-space beam
propagating normally to the PVL plane. This mechanism is highly efficient
for a large range of AM values carried by the impinging PV, with the
only losses attributed to the ohmic dissipation. In addition, our
calculations show that by optimization of the geometrical parameters,
the circular polarization mixing in the outgoing wave can be kept
lower than 15%. As a result, output beams can be theoretically generated
at the wavelength scale in an almost-pure electromagnetic eigenstate.
Interestingly, we also demonstrate that, by reciprocity, the structure
can be exploited in the reverse way as an efficient localized Laguerre–Gaussian
beam-to-plasmonic-vortex coupler, with back-reflected power lower
than 1%.
Figure 1
(a) 3D scheme of the PVL. The geometrical parameters of the spiral
slits include a slit width of 200 nm, pitch of 763 nm, gold thickness
of 150 nm, and Si3N4 thickness of 100 nm. R0, namely the initial radius of the spirals,
is fixed to 4 μm to reduce the effect of direct scattering of
light from the grooves. (b) Scanning electron microscope image of
an example of fabricated structure. (c–e) |E|
maps (vertical cross-section) and E maps (metal surface plots) of the central region of the PVLs
in the case of a PV impinging with topological charge of l = 1 propagating through a flat PVL center (c), scattered by a conical
tip with a zero-basis curvature radius (rc) (d), and by a conical tip with large rc (e). (f) |E| maps in the case of a smoothed conical
tip (same parameters as in (e)) illuminated by a PV with the indicated l values.
(a) 3D scheme of the PVL. The geometrical parameters of the spiral
slits include a slit width of 200 nm, pitch of 763 nm, gold thickness
of 150 nm, and Si3N4 thickness of 100 nm. R0, namely the initial radius of the spirals,
is fixed to 4 μm to reduce the effect of direct scattering of
light from the grooves. (b) Scanning electron microscope image of
an example of fabricated structure. (c–e) |E|
maps (vertical cross-section) and E maps (metal surface plots) of the central region of the PVLs
in the case of a PV impinging with topological charge of l = 1 propagating through a flat PVL center (c), scattered by a conical
tip with a zero-basis curvature radius (rc) (d), and by a conical tip with large rc (e). (f) |E| maps in the case of a smoothed conical
tip (same parameters as in (e)) illuminated by a PV with the indicated l values.We notice that a number
of conical nanotips have already been proposed in combination with
PVL architectures[23−26] but mainly with the purpose of concentrating the axially symmetric l = 0 PV in very localized volumes (nanofocusing).[27] For this purpose, a large curvature radius at
the tip basis is not needed or is even detrimental.[26] Other vertical or horizontal rod-like solutions have been
proposed with the aim to decouple plasmonic vortices to the far-field.[28−30] Most of the studied conical structures consider an abrupt connection
between the antenna basement and the underlying metal surface. In
these architectures, the decoupling takes place by means of the excitation
of one of the antenna electric resonances,[28] whose scattered field pattern is then collected in the far field.
The scattering approach to decoupling PV has, however, severe limitations.
First, the mechanism can be exploited only to decouple axially symmetric
PVs, which have a field maximum in correspondence of the antenna location.
PVs with higher topological charge have a field minimum at the PVL
center; thus, the antenna resonances cannot be excited. Moreover,
PVs can hardly be efficiently decoupled out of the PVL surface, most
of the power is being scattered back again in the form of a PV.The practical exploitation of our plasmonic-vortex-to-free-space
mode matcher, presented here for the first time to the best of our
knowledge, requires a fine control of the shape of such a nontrivial
3D structure, which is mandatory for obtaining the desired effect.
Here, we adopted a powerful technique, sometimes termed as secondary electron lithography.[31−33] This fabrication
procedure proved to enable full control of the shape at the nano-
and microscales, even for exotic 3D nanostructures.[32] This allowed the fabrication of several PVL and tip structures
with excellent matching to the designed profile.In Figure a, we show a 3D scheme
of the proposed structure. A multiple-turn spiral slit is milled on
a 150 nm gold film deposited onto a 100 nm Si3N4 membrane. Its spiral shape is defined byHere, ϕ is the azimuthal
angle, ranging from 0 to 2πN, with N being the number of spiral turns, kSPP is the propagation constant of the SPP mode on a flat gold–air
interface, m is an integer denoting the pitch of
the spiral, and R0 is the distance from
the center to the nearest point of the groove. To maximize the coupling
to the plasmonic vortices, we consider a set of m spirals, each one rotated by 2π/m with respect
to the adjacent ones, in such a way that the radial distance between
two adjacent grooves is λSPP = 2π/kSPP.The other geometrical parameters of the spiral
(slit width and gold thickness) have been tuned to maximize the coupling
efficiency of a circularly polarized plane wave impinging from the
Si3N4side to the SPP modes of the upper gold–air
interface (details are reported in the figure caption). A conical
gold tip, whose profile is reported in the inset of Figure a, is located exactly at the
center of the spiral. A total of three main parameters define the
tip shape: height (h), apex angle (α), and
curvature radii at the basis (rc). The
curvature radius at the tip apex is kept fixed to 10 nm throughout
the paper. As discussed in the experimental details, the adopted fabrication
technique enables us to faithfully reproduce the designed shape (Figure b).We consider
a circularly polarized plane wave impinging normally from the Si3N4side. As has been described in several papers,[8−10,14−16,19] the component of the impinging light electric field
locally orthogonal to the slits efficiently couples to the SPP mode
of the gold–air interface. The plasmonic field launched by
each concentric spiral constructively interferes (thanks to the choice
of the spiral period, λSPP), producing a PV that
radially propagates toward the PVL center. In the absence of a tip,
the PV confined by the spiral grooves forms a standing wave, giving
rise to the characteristic Bessel interference pattern. We use the
finite elements software COMSOL Multiphysics to simulate the electromagnetic
distribution in such a flat PVL (see Figure c). The z component of the
electric field can be expressed analytically, in cylindrical coordinates,
as[10]where kSPP is the wave vector of an SPP propagating on a flat gold–air
interface, J is the
Bessel function of the first kind, and , where k0 = 2π/λ0 is the vacuum wave vector. It can be shown[8−10,14] that the topological charge of a PV is given by the
relation l = m + si, where the spin number si = 1 corresponds to the right-hand and si = −1 to the left-hand circularly polarized
light.When the conical tip is present at the PVL center, the
surface confined electromagnetic mode may couple to the guided mode
propagating along the tip upward. In Figure d,e, we compare the simulations of the same
PV, as shown in Figure c, converging toward two structures having similar conical tips (height h = 6200 nm and an apex angle α = 15°) but with
different curvature radii at the basis. In the case of the negligible
curvature radius (rc → 0), most
of the energy is reflected back, which can be clearly deduced from
the strong fringe modulation of the intensity (see Figure d). This resembles common configurations
presented elsewhere.[23−26] The fraction of the power scattered to the far-field with respect
to the power, incoming at the tip basis (we term this quantity transmittance
hereafter) in this configuration is rather low (less than 10%).This behavior dramatically changes with increasing of the curvature
radius at the tip basis. This is shown in Figure e, where we consider the tip basis curvature
of rc = 1.57 μm. By looking at the
field maps, we now see a smooth intensity pattern close to the metal
surface around the tip, which means the absence of back reflected
SPP at the tip basis. This is also demonstrated by the E field pattern on the metal surface,
which shows perfectly spiraling wave fronts propagating along the
tip. The smoothed tip in this configuration perfectly matches the
PV with the corresponding plasmonic mode of the conical waveguide.
Most of the PV power is finally delivered to the free-space as a z-oriented beam.Figure f reports the |E| maps for the
PVs with l = 0, 2, 3, and 4. As can be seen, for l > 1, the behavior is similar, and the PV are efficiently
decoupled as doughnut-shaped waves propagating in the free space.
The case of l = 0 is an interesting exception. This
PV propagates to the end of the tip and is almost fully reflected
back, which can be deduced by observing the interference pattern along
the metal surface.A study of the PV transmittance as a function
of l for different values of rc is summarized in the Figure a. It is clearly seen that the increasing of rc leads to a gradual improvement of the out-coupling
efficiencies of the PVs, which can reach values as high as 90%, even
for large l values. The only losses can be ascribed
to the metal absorption. We notice, however, that the coupling of
the PV with l = 0 to the far field is always very poor.
Figure 2
(a) Fraction of the PV light power transmitted to the
air domain as a function of the PV topological charge, l, for increasing values of rc. (b) Cutoff
radii of the plasmonic modes propagating along the tip, calculated
by solution of the exact cylindrical mode dispersion equation (red)
compared with those extracted from the finite elements simulation
(green circles); the blue asterisks denotes the primary ring radii
of PVs propagating on a flat gold–air surface; the horizontal
dashed lines mark, respectively, the inner tip radius before the smoothing,
650 nm, and the maximum tip radius, 2200 nm; the inset shows an example
of an electric field norm map calculated in a model of a semi-infinite
gold tip.
(a) Fraction of the PV light power transmitted to the
air domain as a function of the PV topological charge, l, for increasing values of rc. (b) Cutoff
radii of the plasmonic modes propagating along the tip, calculated
by solution of the exact cylindrical mode dispersion equation (red)
compared with those extracted from the finite elements simulation
(green circles); the blue asterisks denotes the primary ring radii
of PVs propagating on a flat gold–air surface; the horizontal
dashed lines mark, respectively, the inner tip radius before the smoothing,
650 nm, and the maximum tip radius, 2200 nm; the inset shows an example
of an electric field norm map calculated in a model of a semi-infinite
gold tip.To understand the PV propagation
along the cone and their final decoupling, we consider the modes of
a conducting cylindrical waveguide placed along the z-axis, whose radius, ρ, progressively decreases with z. Their electric field can be expressed as[34,35]where the subscript i = 1
or 2 and denotes the region outside and inside the cylinder, respectively;
β is the complex propagation constant of the mode; and k is the transverse wave
vector, such that εk02 = β2 + k2, with k0 = ω/c being the vacuum wave vector and ε1 = 1, ε2 = −24.1 + 1.7i being the relative permittivities of vacuum and gold.[36] The mode amplitude Ẽ (kρ)
as well as β can be obtained from the solution of the Helmholtz
equation in cylindrical coordinates in the metal and air domains,
respectively, via the imposition of the continuity of the tangential
components of the E and H fields at the
metal surface. This procedure yields a well-known dispersion equation,[35] which we solved numerically. Details of the
real and imaginary parts of the modes effective index as a function
of the cylinder radius are given in the Supporting Information.As extensively discussed in the literature,[35] the mode with l = 0 has a diverging
mode index and experiences zero group velocity close to the ρ
= 0. This is the reason why such conical structures have been widely
utilized for nanofocusing purposes.[26,27] In the case
of adiabatic tapering, corresponding to the small variations of the
plasmon wavenumber on the scale of a plasmon wavelength, the mode
progressively slows to almost a full stop, leading to a giant concentration
of energy at the nanoscale volume.[26] In
this case, a zero transmittance to the far field would be expected.
In our case, the tip aperture is small but non-negligible, so the
abrupt termination results in reflections from the tip end, clearly
visible in Figure f, and in a partial scattering to the far field. The latter is the
cause of the low transmittance calculated for l =
0 in Figure a.The l = 1 mode also needs a separate discussion.
In this case, the group velocity adiabatically approaches c, and its propagation constant tends to k0 as ρ → 0.[35] This
mode is, therefore, guided to the tip end, where it efficiently decouples
to the free space. The perfect momentum matching in this case assures
no back-reflections, and most of the energy is beamed out. Apparently
with this mode, one obtains a Gaussian beam- like source of radiation
rather than a localization of the energy at the tip end, which is
important in applications where high optical throughput is needed.All other modes, l >1, exist in a bound form
only for ρ larger than some l-dependent cutoff
value, at which the modal loss vanishes (Im(β) = 0).[37] To verify that such a mode conversion
mechanisms takes place along our conical tip, which has a small but
non-negligible aperture of α = 15°, we simulate just a
portion of a very long metal tip, exciting the lth
mode at the basis boundary (Figure b inset). This enables us to exclude from the analysis
the effects of the finite length of the tip, thus allowing the study
of arbitrarily high l values. We empirically estimate
the modes detaching points by considering the points at which the
electric field norm along the metal surface reaches its maximum. The
corresponding radii for l from 1 to 7 are marked
in Figure b with green
dots. As can be seen, the cutoff values obtained from solution of
the exact dispersion equation (red asterisks) are in good agreement
with the numerical simulation. We notice that the tip we consider
(h = 6200 nm, rc = 1570
nm) has a maximum radius of about 2.2 μm, at the beginning of
the smoothed part, while the tip radius at the fillet end is just
650 nm (these radii are marked with horizontal dashed lines in Figure b). This latter is
the radius at which the tip slope effectively starts to be equal to
α/2 = 7.5°. This radius is just larger than the cutoff
of l = 2 mode. Nonetheless, a high transmittance
is predicted for all modes up to l = 6, as can be
seen in Figure a (black
line). For these modes, the large curvature radius at the basis ensures
a smooth transition between the plasmon modes and the free propagating
waves in air. For l > 6, transmittance rapidly
drops (Figure a, yellow
line), becoming zero for l > 15. As a matter of
fact, we notice that when l > 6, the cutoff radius
is larger than the maximum tip radius. For l up to
16, however, we observe that the first maximum of the Bessel interference
pattern that would arise in the absence of tip (sometimes called the
primary ring;[9] blue line in Figure b) occurs at a radius smaller
than the maximum tip radius. This enables an interaction with the
tip basis, which determines a partial decoupling of the PV to the
free space. For l > 16, instead, the primary ring
radius is larger than the maximum tip radius, and therefore, the PV
does not interact with the tip at all, resulting in a situation similar
to a flat PVL, like in Figure c. Accordingly, in this situation, the decoupled power is
zero. To increase the maximum lth mode interacting
with the tip, a higher tip with the same curvature radius at the basis
can be prepared (as can be evinced from Figure b).Once the lth mode
detaches from the tip, it propagates in air as a wave with the unique
spatial phase-structuring. The radial polarization of the PV at the
tip surface collapses in the free space into the scalar components
of two opposite circular polarizations, E± = E − isoZH,[20] carrying OAM of lo = l – so = l ∓
1, where the OAM of the PV is l = m + si = m ± 1; si is the incident spin number and so is the spin of the outcoupled light. We can summarize
the expected OAM content of the output cross-circular polarization
components in Table .[20]
Table 1
Topological Charges
of the Outcoupled Beam Depending on the Incident and the Emerging
Polarization State
Table 1
si = +1
si = −1
so = +1
m
m –
2
so = −1
m + 2
m
As has been stressed
elsewhere,[38] the process of the impinging
light scattering results in the appearance of some amount of a spin-flip
component (that is, the light of opposite handedness with respect
to the incident one). This mix of the output polarization states can
be large and depends, besides the geometry of the structure, on particular
symmetries of Maxwell’s equations.[39,40] In this regard, we notice that our structure behaves as a mode matcher rather than a scatterer. Specifically, the
coupling of the incident circularly polarized light to PV followed
by its guidance to the tip apex incorporates the 3D transformation
of the electromagnetic fields. The surface curvature, combined with
an effective index change along the tip, forces the emerging spin
to be s0 = sgn(l).[40] In other words, for positive topological charges
of the PVs, the tip emits the light with an almost-pure spin state
of so = 1. The tip profile we present
has been optimized to simultaneously maximize, for l ranging from 1 to 4, both the tip transmittance and the polarization
contrast. The latter is defined as Q = 1 – P+/P–, with P+ and P– being
the light powers decoupled by the tip with right and left circular
polarization state, respectively. A plot of transmittance and Q for the first l values is reported in Figure a. As can be seen, Q remains higher than 83% for l = 1 to
4. For more details about the tip parameter optimization, we remand
attention to the Supporting Information.
Figure 3
(a) Polarization contrast (red) and tip transmittance (blue) as a
function of the PV topological charge, l. (b) Simulated
|E| field profiles for various l (colored
lines) taken at a horizontal cross-section 1 μm above the tip
compared with the corresponding fit curves, obtained by using eq . (c) Simulated divergences
of the beams in the case of the finite smoothed tip (blue line) compared
to the semi-infinite one (green). (d) Examples of simulations of coupling
of a focused Laguerre–Gaussian beam to the plasmonic vortex
by coaxial illumination of the tip from above. As indicated in the
figure, the beams have lo = 0 and so = 1 (Gaussian beam) and lo = 1 and so = 1 (Laguerre–Gaussian
beam).
(a) Polarization contrast (red) and tip transmittance (blue) as a
function of the PV topological charge, l. (b) Simulated
|E| field profiles for various l (colored
lines) taken at a horizontal cross-section 1 μm above the tip
compared with the corresponding fit curves, obtained by using eq . (c) Simulated divergences
of the beams in the case of the finite smoothed tip (blue line) compared
to the semi-infinite one (green). (d) Examples of simulations of coupling
of a focused Laguerre–Gaussian beam to the plasmonic vortex
by coaxial illumination of the tip from above. As indicated in the
figure, the beams have lo = 0 and so = 1 (Gaussian beam) and lo = 1 and so = 1 (Laguerre–Gaussian
beam).Finally, we characterize the propagating
waves decoupled by the tip in terms of divergence and intensity profile.
It is important to underline that, unlike other configurations presented
in literature,[28−30] in this case, what is transmitted to the far field
is a well-defined beam with a single intensity lobe. Figure b reports the electric field
norm profiles for l = 1 to 5 calculated on a horizontal
cross-section 1 μm above the tip. We notice that profiles are
well-fitted by Laguerre–Gaussian beam shapes (dashed black
lines), namelywith lo = l – so being the OAM of the outgoing wave, w(z) = w0[1
+ (z/zR)0.5], zR = πw02/λ0 being the Rayleigh range and adopting as parameters a and z and the beam waist, w0. The inset of Figure b shows the far-field polar plots for each l. Clearly, the peak intensities are found within a cone of maximum
40° half-aperture. Figure c presents the beams divergences (i.e., the angles from the
normal at which the intensity drops to 1/e times
the peak value) for l = 1 to 5. We compare the cases
of finite-height smoothed tips and the infinite tip. As can be seen,
the divergences are similar only for l = 1 and 2
because for these l values, in both the realistic
and idealized tip models, the PVs propagate along the tapered part
of the tip before detaching. Nonetheless, for all l from 2 to 5, the beam divergences are lower than about 60°.
Therefore, the output beams are readily measurable by standard microscope
objectives, (an angular apertures of 60° corresponds to numerical
apertures of 0.866). Interestingly, these results suggest that the
smoothed conical structure can be exploited also as a perfect Laguerre–Gaussian
beam-to-plasmonic-vortex converter. As an example, in Figure d, we simulate the illumination
of the tip by normally impinging circularly polarized focused Laguerre–Gaussian
beams with lo = 0, 1 setting the beam
parameters to those ones obtained from the fits of the corresponding
outgoing waves produced by PV decoupling. As can be seen, the electric
field norm distributions show a very smooth coupling to the conical
tip modes and, finally, to the PV modes. The calculated back-reflections
are lower than 1%, while the power delivered to PVs at the tip base
is 76% for lo = 0 and 84% for lo = 1.To prove the aforementioned properties
of beaming of helical light by means of our adiabatically tapered
tip, we provide the experimental demonstrations of the presented analytical
and numerical simulations. The sample was illuminated from the bottom
with a 20 mW CW single mode pigtailed laser at λ0 = 780 nm. Its spatially filtered and collimated beam was normally
incident from the substrate side on the spiral grooves surrounding
the tips, and an additional optical objective (Olympus LMPLANFL 100×,
NA 0.8) was used to produce an image the tips at CMOS camera (Hamamatsu
Orca R2-cooled CCD). According to our simulations, the NA of the imaging
objective is large enough to capture the beaming light distribution
of up to lo = 5. For higher topological
charges, a near-field scanning microscopy might be used due to the
strong angular deviation of the scattered light. We used a set of
a linear polarizer (LP) followed by a quarter-wave plate (QWP) to
tune the incident polarization state and an additional set of QWP
and an LP to analyze the emerging polarization.For the sample
fabrication, an optimized procedure was developed (fully described
in the Supporting Information). The fabrication
of such high tips with arbitrary profiles cannot be performed by means
of the well-known electron-beam-induced deposition (EBID)[41] because the process is not stable enough. This
limitation was solved by using an approach already used in high-aspect-ratio
3D plasmonic structure fabrication.[31−33] Briefly, the backbone
of the 6.2 μm high tip was prepared by means of focused ion
beam (FIB) (FEI Novalab 600i) exposure on a thick layer of S1813 resist
spun on a thin (100 nm) Si3N4 membrane. A 150
nm gold layer was deposited on the membrane, and then the PVL slit
patterns with the geometrical vortex topological charges m ranging from 0 to 3 were inscribed on the Au layer using the FIB.
An example of the fabricated nanotip with the surrounding PVL is reported
in Figure b. A scanning
electron microscopy (SEM) image of the PVL with the geometric vortex
topological charge of m = 3 is illustrated. In the Supporting Information, additional examples of
fabricated samples can be seen with details on the 3D profile, providing
evidence that the obtained tip shape almost perfectly matches the
designed one.Figure demonstrates the intensity distributions captured by our
setup above the structures with m = 0, 1, 2, or 3.
We arrange the results for different polarization states in the order
prescribed by the Table . As expected, our camera captures helical field distributions with
topological charges up to lo = +5. Due
to unavoidable imperfections, the singularity of the beam is split
into fundamental first-order singularities, providing a convenient
way to verify the resultant OAM of the emerging beam, which nicely
corresponds to the prediction given in the Table . We note that, as expected, the PVLs with m = 0 and m = 2 produce point-like emission
expressed as an Airy distribution. In some panels, we added red arrows
to guide the eye to the singular points. For m = 3 for (si,so) = (+1,–1), the beam divergence approaches our imaging limit,
and therefore, the singularities are not clearly visible; however,
the large primary ring is a clear signature for its high OAM. The
helicity conservation effect can be clearly deduced from the PVL structure
with m = 0. This structure has a circular symmetry;
therefore, the plasmonic vortex topological charge is l = si. Accordingly, as stated before,
the emerging spin state, s0 = sgn(l) = si. We note that in the
experiment, other sources of helicity change, such as scattering from
the spiral rings and direct transmission, would limit the polarization
contrast to lower values than the ones predicted by our simulations.
However, the measured intensity distribution is fully consistent with
this selection rule, as one can clearly see the undoubtedly high contrast
between the pictures taken with the same polarizer–analyzer
state (diagonal) and the ones taken with crossed polarizers (antidiagonal).
Due to specific experiment conditions, the results for higher order
PVLs presented in Figure do not allow a visual estimation of the polarization contrast,
which is one of the topics of our current research.
Figure 4
Far-field intensity distributions
measured using combinations of circular input polarizers and output
analyzers. The images are arranged according to the incident and emerging
polarization states (si and so, respectively) as in Table . The expected topological charges of the
far-field beams, lo, are reported in each
image, and the red arrows are added to guide the eye to the singularity
points.
Far-field intensity distributions
measured using combinations of circular input polarizers and output
analyzers. The images are arranged according to the incident and emerging
polarization states (si and so, respectively) as in Table . The expected topological charges of the
far-field beams, lo, are reported in each
image, and the red arrows are added to guide the eye to the singularity
points.In our last experiment, we utilized
the fabricated tips as the plasmonic vortex generator in the near
field. To measure this, we slightly modify the fabrication process
by preparing a tip on top of a 60 nm thick gold layer without any
grating around it. We illuminate the tip by a slightly focused laser
beam (20× objective) and image the leakage radiation by using
an oil-immersion 100× objective (NA 1.25). This leakage radiation
microscopy system (LRM) provides us with a direct image of the plasmonic
modes excited at the metal–air interface.[42]Figure demonstrates the experimental setup along with the measured results.
As can be seen from Figure b, the stand-alone tip produces plasmonic vortices with l = ±1, which yields in the far field structured waves
with lo = 0 and ± 2, as expected
from ideally center symmetric geometry. We verified that the spatial
frequency of the measured disturbance, k = 8.45,
corresponds to the expected plasmonic wavelength. This confirms that
our system indeed captures the near-field surface waves distribution.
Figure 5
Near-field
PV generation by a nanotip. (a) Scheme of the LRM setup used to measure
the near field. Polarization components LP and QWP were used to tune
and analyze the polarization, a 20× objective (Obj1) was used
to prefocus the beam on the tip, an oil immersion 1.25NA objective
(Obj2) extracted the leakage radiation, and a set of the lenses (L1–L3)
was used to image the SP distribution. (b) Measured LRM in the case
of a tip fabricated with a 30 nm gold coating layer.
Near-field
PV generation by a nanotip. (a) Scheme of the LRM setup used to measure
the near field. Polarization components LP and QWP were used to tune
and analyze the polarization, a 20× objective (Obj1) was used
to prefocus the beam on the tip, an oil immersion 1.25NA objective
(Obj2) extracted the leakage radiation, and a set of the lenses (L1–L3)
was used to image the SP distribution. (b) Measured LRM in the case
of a tip fabricated with a 30 nm gold coating layer.In summary, we presented a plasmonic vortex lens
structure able to couple a circularly polarized light to a plasmonic
vortex and to efficiently transmit it to the far-field by means of
a smoothed-cone tip placed at its center. The large curvature radius
at the cone basis is shown to play a crucial role in enabling an adiabatic
coupling of the PV propagating on the flat metal surface to the plasmonic
modes of the metal tip, whose tapering, in turn, enables an adiabatic
match to the propagating waves in free space. This particular nontrivial
geometry has been faithfully experimentally fabricated by the secondary
electron lithography technique. The optical characterization revealed
that phase-structured beams were successfully transmitted by the tip
up to OAM l0 = 5. Finally, our simulations
have shown that this structure can work as an excellent coupler of
focused Laguerre–Gaussian beam to PVs. A proof of concept measurement
in this illumination condition has been shown by adopting a leakage
radiation microscopy setup.We believe that such architecture
can be a key element for the realization of compact focused-beams-to-plasmonic-wave
couplers, elements that are highly desirable to fully exploit plasmonic
technologies in practical applications, such as sensing, light manipulation
in flat guided optics, optical tweezing, etc. On the other side, a
scattering-free, highly directional PV read-out element could be also
extremely valuable, enabling us to directly visualize any near-field
coherent azimuthal interference taking place at the center of a PVL.
Thanks to the flexibility of secondary electron lithography (as demonstrated
elsewhere),[31] complete control of the tip
shape can be obtained, enabling us to finely tune the coupling–decoupling
capability of the tip, thus making it interesting for a large number
of applications. For example, smaller tips can be used to decouple
PVs produced by simple bull’s eye structures, while a higher
tip can enable far-field access to arbitrary high-OAM-carrying PVs.