Literature DB >> 26848136

On the relationship between aerosol model uncertainty and radiative forcing uncertainty.

Lindsay A Lee1, Carly L Reddington1, Kenneth S Carslaw2.   

Abstract

The largest uncertainty in the historical radiative forcing of climate is caused by the interaction of aerosols with clouds. Historical forcing is not a directly measurable quantity, so reliable assessments depend on the development of global models of aerosols and clouds that are well constrained by observations. However, there has been no systematic assessment of how reduction in the uncertainty of global aerosol models will feed through to the uncertainty in the predicted forcing. We use a global model perturbed parameter ensemble to show that tight observational constraint of aerosol concentrations in the model has a relatively small effect on the aerosol-related uncertainty in the calculated forcing between preindustrial and present-day periods. One factor is the low sensitivity of present-day aerosol to natural emissions that determine the preindustrial aerosol state. However, the major cause of the weak constraint is that the full uncertainty space of the model generates a large number of model variants that are equally acceptable compared to present-day aerosol observations. The narrow range of aerosol concentrations in the observationally constrained model gives the impression of low aerosol model uncertainty. However, these multiple "equifinal" models predict a wide range of forcings. To make progress, we need to develop a much deeper understanding of model uncertainty and ways to use observations to constrain it. Equifinality in the aerosol model means that tuning of a small number of model processes to achieve model-observation agreement could give a misleading impression of model robustness.

Keywords:  aerosol−cloud interaction; model constraint; uncertainty analysis

Year:  2016        PMID: 26848136      PMCID: PMC4889342          DOI: 10.1073/pnas.1507050113

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  8 in total

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Authors:  Anja Schmidt; Bart Ostro; Kenneth S Carslaw; Marjorie Wilson; Thorvaldur Thordarson; Graham W Mann; Adrian J Simmons
Journal:  Proc Natl Acad Sci U S A       Date:  2011-09-19       Impact factor: 11.205

2.  Global estimate of aerosol direct radiative forcing from satellite measurements.

Authors:  Nicolas Bellouin; Olivier Boucher; Jim Haywood; M Shekar Reddy
Journal:  Nature       Date:  2005-12-22       Impact factor: 49.962

3.  Strong present-day aerosol cooling implies a hot future.

Authors:  Meinrat O Andreae; Chris D Jones; Peter M Cox
Journal:  Nature       Date:  2005-06-30       Impact factor: 49.962

4.  Large contribution of natural aerosols to uncertainty in indirect forcing.

Authors:  K S Carslaw; L A Lee; C L Reddington; K J Pringle; A Rap; P M Forster; G W Mann; D V Spracklen; M T Woodhouse; L A Regayre; J R Pierce
Journal:  Nature       Date:  2013-11-07       Impact factor: 49.962

5.  Satellite methods underestimate indirect climate forcing by aerosols.

Authors:  Joyce E Penner; Li Xu; Minghuai Wang
Journal:  Proc Natl Acad Sci U S A       Date:  2011-08-01       Impact factor: 11.205

6.  Occurrence of pristine aerosol environments on a polluted planet.

Authors:  Douglas S Hamilton; Lindsay A Lee; Kirsty J Pringle; Carly L Reddington; Dominick V Spracklen; Kenneth S Carslaw
Journal:  Proc Natl Acad Sci U S A       Date:  2014-12-15       Impact factor: 11.205

7.  Atmospheric science. Climate effects of aerosol-cloud interactions.

Authors:  Daniel Rosenfeld; Steven Sherwood; Robert Wood; Leo Donner
Journal:  Science       Date:  2014-01-24       Impact factor: 47.728

8.  From aerosol-limited to invigoration of warm convective clouds.

Authors:  Ilan Koren; Guy Dagan; Orit Altaratz
Journal:  Science       Date:  2014-06-06       Impact factor: 47.728

  8 in total
  7 in total

1.  Improving our fundamental understanding of the role of aerosol-cloud interactions in the climate system.

Authors:  John H Seinfeld; Christopher Bretherton; Kenneth S Carslaw; Hugh Coe; Paul J DeMott; Edward J Dunlea; Graham Feingold; Steven Ghan; Alex B Guenther; Ralph Kahn; Ian Kraucunas; Sonia M Kreidenweis; Mario J Molina; Athanasios Nenes; Joyce E Penner; Kimberly A Prather; V Ramanathan; Venkatachalam Ramaswamy; Philip J Rasch; A R Ravishankara; Daniel Rosenfeld; Graeme Stephens; Robert Wood
Journal:  Proc Natl Acad Sci U S A       Date:  2016-05-24       Impact factor: 11.205

2.  AEROSOL-CLOUD-METEOROLOGY INTERACTION AIRBORNE FIELD INVESTIGATIONS: Using Lessons Learned from the U.S. West Coast in the Design of ACTIVATE off the U.S. East Coast.

Authors:  Armin Sorooshian; Bruce Anderson; Susanne E Bauer; Rachel A Braun; Brian Cairns; Ewan Crosbie; Hossein Dadashazar; Glenn Diskin; Richard Ferrare; Richard C Flagan; Johnathan Hair; Chris Hostetler; Haflidi H Jonsson; Mary M Kleb; Hongyu Liu; Alexander B MacDonald; Allison McComiskey; Richard Moore; David Painemal; Lynn M Russell; John H Seinfeld; Michael Shook; William L Smith; Kenneth Thornhill; George Tselioudis; Hailong Wang; Xubin Zeng; Bo Zhang; Luke Ziemba; Paquita Zuidema
Journal:  Bull Am Meteorol Soc       Date:  2019-08-28       Impact factor: 8.766

3.  Reducing the aerosol forcing uncertainty using observational constraints on warm rain processes.

Authors:  Johannes Mülmenstädt; Christine Nam; Marc Salzmann; Jan Kretzschmar; Tristan S L'Ecuyer; Ulrike Lohmann; Po-Lun Ma; Gunnar Myhre; David Neubauer; Philip Stier; Kentaroh Suzuki; Minghuai Wang; Johannes Quaas
Journal:  Sci Adv       Date:  2020-05-29       Impact factor: 14.136

4.  The hemispheric contrast in cloud microphysical properties constrains aerosol forcing.

Authors:  Isabel L McCoy; Daniel T McCoy; Robert Wood; Leighton Regayre; Duncan Watson-Parris; Daniel P Grosvenor; Jane P Mulcahy; Yongxiang Hu; Frida A-M Bender; Paul R Field; Kenneth S Carslaw; Hamish Gordon
Journal:  Proc Natl Acad Sci U S A       Date:  2020-07-27       Impact factor: 11.205

5.  Statistical Emulation of Winter Ambient Fine Particulate Matter Concentrations From Emission Changes in China.

Authors:  Luke Conibear; Carly L Reddington; Ben J Silver; Ying Chen; Christoph Knote; Stephen R Arnold; Dominick V Spracklen
Journal:  Geohealth       Date:  2021-05-01

6.  Sensitivity of Air Pollution Exposure and Disease Burden to Emission Changes in China Using Machine Learning Emulation.

Authors:  Luke Conibear; Carly L Reddington; Ben J Silver; Ying Chen; Christoph Knote; Stephen R Arnold; Dominick V Spracklen
Journal:  Geohealth       Date:  2022-06-01

7.  Predicting secondary organic aerosol phase state and viscosity and its effect on multiphase chemistry in a regional-scale air quality model.

Authors:  Ryan Schmedding; Quazi Z Rasool; Yue Zhang; Havala O T Pye; Haofei Zhang; Yuzhi Chen; Jason D Surratt; Felipe D Lopez-Hilfiker; Joel A Thornton; Allen H Goldstein; William Vizuete
Journal:  Atmos Chem Phys       Date:  2020-07-16       Impact factor: 6.133

  7 in total

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