Literature DB >> 26633125

Redox-Dependent Franck-Condon Blockade and Avalanche Transport in a Graphene-Fullerene Single-Molecule Transistor.

Chit Siong Lau1, Hatef Sadeghi2, Gregory Rogers1, Sara Sangtarash2, Panagiotis Dallas1, Kyriakos Porfyrakis1, Jamie Warner1, Colin J Lambert2, G Andrew D Briggs1, Jan A Mol1.   

Abstract

We report transport measurements on a graphene-fullerene single-molecule transistor. The device architecture where a functionalized C60 binds to graphene nanoelectrodes results in strong electron-vibron coupling and weak vibron relaxation. Using a combined approach of transport spectroscopy, Raman spectroscopy, and DFT calculations, we demonstrate center-of-mass oscillations, redox-dependent Franck-Condon blockade, and a transport regime characterized by avalanche tunnelling in a single-molecule transistor.

Entities:  

Keywords:  Franck−Condon blockade; Single-molecule electronics; avalanche transport; electron-vibron coupling; graphene

Year:  2015        PMID： 26633125     DOI： 10.1021/acs.nanolett.5b03434

Source DB:  PubMed          Journal:  Nano Lett        ISSN： 1530-6984            Impact factor:   11.189


  7 in total

1.  Chemical Control and Spectral Fingerprints of Electronic Coupling in Carbon Nanostructures.

Authors:  Jacek Kłos; Mijin Kim; Millard H Alexander; YuHuang Wang
Journal:  J Phys Chem C Nanomater Interfaces       Date:  2016-12-07       Impact factor: 4.126

2.  Stable anchoring chemistry for room temperature charge transport through graphite-molecule contacts.

Authors:  Alexander V Rudnev; Veerabhadrarao Kaliginedi; Andrea Droghetti; Hiroaki Ozawa; Akiyoshi Kuzume; Masa-Aki Haga; Peter Broekmann; Ivan Rungger
Journal:  Sci Adv       Date:  2017-06-09       Impact factor: 14.136

3.  Distinguishing Lead and Molecule States in Graphene-Based Single-Electron Transistors.

Authors:  Pascal Gehring; Jakub K Sowa; Jonathan Cremers; Qingqing Wu; Hatef Sadeghi; Yuewen Sheng; Jamie H Warner; Colin J Lambert; G Andrew D Briggs; Jan A Mol
Journal:  ACS Nano       Date:  2017-04-21       Impact factor: 15.881

4.  Understanding resonant charge transport through weakly coupled single-molecule junctions.

Authors:  James O Thomas; Bart Limburg; Jakub K Sowa; Kyle Willick; Jonathan Baugh; G Andrew D Briggs; Erik M Gauger; Harry L Anderson; Jan A Mol
Journal:  Nat Commun       Date:  2019-10-11       Impact factor: 14.919

5.  Electrochemical control of the single molecule conductance of a conjugated bis(pyrrolo)tetrathiafulvalene based molecular switch.

Authors:  Luke J O'Driscoll; Joseph M Hamill; Iain Grace; Bodil W Nielsen; Eman Almutib; Yongchun Fu; Wenjing Hong; Colin J Lambert; Jan O Jeppesen
Journal:  Chem Sci       Date:  2017-06-23       Impact factor: 9.825

Review 6.  Hybrids of Fullerenes and 2D Nanomaterials.

Authors:  Muqing Chen; Runnan Guan; Shangfeng Yang
Journal:  Adv Sci (Weinh)       Date:  2018-09-02       Impact factor: 16.806

Review 7.  Functional Redox-Active Molecular Tunnel Junctions.

Authors:  Yingmei Han; Christian A Nijhuis
Journal:  Chem Asian J       Date:  2020-10-14
  7 in total

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