Literature DB >> 26389651

Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO3 Thin Films.

Frank Chen1,2, John Goodfellow1,3, Shi Liu4, Ilya Grinberg4, Matthias C Hoffmann5, Anoop R Damodaran6, Yi Zhu7, Peter Zalden1, Xiaohang Zhang8, Ichiro Takeuchi8, Andrew M Rappe4, Lane W Martin6,9, Haidan Wen7, Aaron M Lindenberg1,3,10.   

Abstract

Terahertz pulses are applied as an all-optical bias to ferroelectric thin-film BiFeO3 while monitoring the time-dependent ferroelectric polarization through its nonlinear optical response. Modulations in the intensity of the second harmonic light generated by the film correspond to on-off ratios of 220× gateable on femtosecond timescales. Polarization modulations comparable to the built-in static polarization are observed.
© 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Entities:  

Keywords:  ferroelectrics; nonlinear optical properties; terahertz modulators; ultra-fast

Year:  2015        PMID: 26389651     DOI: 10.1002/adma.201502975

Source DB:  PubMed          Journal:  Adv Mater        ISSN: 0935-9648            Impact factor:   30.849


  4 in total

1.  Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3.

Authors:  M Kozina; T van Driel; M Chollet; T Sato; J M Glownia; S Wandel; M Radovic; U Staub; M C Hoffmann
Journal:  Struct Dyn       Date:  2017-05-03       Impact factor: 2.920

2.  THz Electric Field-Induced Second Harmonic Generation in Inorganic Ferroelectric.

Authors:  Kirill A Grishunin; Nikita A Ilyin; Natalia E Sherstyuk; Elena D Mishina; Alexey Kimel; Vladimir M Mukhortov; Andrey V Ovchinnikov; Oleg V Chefonov; Mikhail B Agranat
Journal:  Sci Rep       Date:  2017-04-06       Impact factor: 4.379

3.  Ultrafast electron-phonon coupling and photo-induced strain in the morphotropic phase boundary of BixDy1-xFeO3 films.

Authors:  Zeyu Zhang; Lu You; Juan Du; Junling Wang; Zuanming Jin; Guohong Ma; Yuxin Leng
Journal:  Sci Rep       Date:  2018-02-19       Impact factor: 4.379

4.  Ultrafast polarization control by terahertz fields via π-electron wavefunction changes in hydrogen-bonded molecular ferroelectrics.

Authors:  T Miyamoto; D Hata; T Morimoto; H Yamakawa; N Kida; T Terashige; K Iwano; H Kishida; S Horiuchi; H Okamoto
Journal:  Sci Rep       Date:  2018-10-09       Impact factor: 4.379

  4 in total

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