Self-assembly of the decagonal quasicrystalline order in simple three-dimensional systems.

Using molecular dynamics simulations we show that a one-component system can be driven to a three-dimensional decagonal (10-fold) quasicrystalline state just by purely repulsive, isotropic and monotonic interaction pair potential with two characteristic length scales; no attraction is needed. We found that self-assembly of a decagonal quasicrystal from a fluid can be predicted by two dimensionless effective parameters describing the fluid structure. We demonstrate stability of the results under changes of the potential by obtaining the decagonal order for three particle systems with different interaction potentials, both purely repulsive and attractive, but with the same values of the effective parameters. Our results suggest that soft matter quasicrystals with decagonal symmetry can be experimentally observed for the same systems demonstrating the dodecagonal order for an appropriate tuning of the effective parameters.