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Literature DB >> 25967883

Versatile Electrochemical C-H Amination via Zincke Intermediates.

Abstract

Simply by applying electricity, the amination reaction of a broad variety of arenes, heteroarenes, and benzylic substrates is achieved. Pyridine serves as the nitrogen source and the intermediate cationic species are well-protected from over-oxidation.

Entities: Chemical

Keywords: amination; electrochemistry; oxidative coupling; sustainable chemistry; synthetic methods

Mesh：

Substances：
Carbon
Copper
Hydrogen

Year: 2015 PMID： 25967883 DOI： 10.1002/anie.201502638

Source DB: PubMed Journal: Angew Chem Int Ed Engl ISSN： 1433-7851 Impact factor: 15.336

Keyword Cloud
Cited

15 in total

1. Electrochemically Enabled, Nickel-Catalyzed Amination.

Authors: Chao Li; Yu Kawamata; Hugh Nakamura; Julien C Vantourout; Zhiqing Liu; Qinglong Hou; Denghui Bao; Jeremy T Starr; Jinshan Chen; Ming Yan; Phil S Baran
Journal: Angew Chem Int Ed Engl Date: 2017-09-14 Impact factor: 15.336

2. Practical Electrochemical Anodic Oxidation of Polycyclic Lactams for Late Stage Functionalization.

Authors: Kevin J Frankowski; Ruzhang Liu; Gregory L Milligan; Kevin D Moeller; Jeffrey Aubé
Journal: Angew Chem Int Ed Engl Date: 2015-09-01 Impact factor: 15.336

3. Metal-Free Electrochemical Synthesis of Sulfonamides Directly from (Hetero)arenes, SO₂ , and Amines.

Authors: Stephan P Blum; Tarik Karakaya; Dieter Schollmeyer; Artis Klapars; Siegfried R Waldvogel
Journal: Angew Chem Int Ed Engl Date: 2021-02-02 Impact factor: 15.336

4. Electrosynthesis and electrochemistry.

Authors: Siegfried R Waldvogel
Journal: Beilstein J Org Chem Date: 2015-06-02 Impact factor: 2.883

5. Solvent-Dependent Facile Synthesis of Diaryl Selenides and Biphenols Employing Selenium Dioxide.

Authors: Thomas Quell; Michael Mirion; Dieter Schollmeyer; Katrin M Dyballa; Robert Franke; Siegfried R Waldvogel
Journal: ChemistryOpen Date: 2015-12-11 Impact factor: 2.911

Review 6. Electrifying Organic Synthesis.

Authors: Anton Wiebe; Tile Gieshoff; Sabine Möhle; Eduardo Rodrigo; Michael Zirbes; Siegfried R Waldvogel
Journal: Angew Chem Int Ed Engl Date: 2018-03-07 Impact factor: 15.336

Versatile Electrochemical C-H Amination via Zincke Intermediates.

1. Electrochemically Enabled, Nickel-Catalyzed Amination.

2. Practical Electrochemical Anodic Oxidation of Polycyclic Lactams for Late Stage Functionalization.

3. Metal-Free Electrochemical Synthesis of Sulfonamides Directly from (Hetero)arenes, SO₂ , and Amines.

4. Electrosynthesis and electrochemistry.

5. Solvent-Dependent Facile Synthesis of Diaryl Selenides and Biphenols Employing Selenium Dioxide.

Review 6. Electrifying Organic Synthesis.

7. Phenothiazinimides: Atom-Efficient Electrophilic Amination Reagents.

8. Charged Tags for the Identification of Oxidative Drug Metabolites Based on Electrochemistry and Mass Spectrometry.

Review 9. Modern Electrochemical Aspects for the Synthesis of Value-Added Organic Products.

10. Metal- and Reagent-Free Electrochemical Synthesis of Alkyl Arylsulfonates in a Multi-Component Reaction.