Literature DB >> 25706329

Giant photoluminescence blinking of perovskite nanocrystals reveals single-trap control of luminescence.

Yuxi Tian1, Aboma Merdasa, Maximilian Peter, Mohamed Abdellah, Kaibo Zheng, Carlito S Ponseca, Tõnu Pullerits, Arkady Yartsev, Villy Sundström, Ivan G Scheblykin.   

Abstract

Fluorescence super-resolution microscopy showed correlated fluctuations of photoluminescence intensity and spatial localization of individual perovskite (CH3NH3PbI3) nanocrystals of size ∼200 × 30 × 30 nm(3). The photoluminescence blinking amplitude caused by a single quencher was a hundred thousand times larger than that of a typical dye molecule at the same excitation power density. The quencher is proposed to be a chemical or structural defect that traps free charges leading to nonradiative recombination. These trapping sites can be activated and deactivated by light.

Entities:  

Keywords:  Perovskite; blinking; charge trapping; photoluminescence; single molecule spectroscopy; super-resolution microscopy

Mesh:

Substances:

Year:  2015        PMID: 25706329     DOI: 10.1021/nl5041397

Source DB:  PubMed          Journal:  Nano Lett        ISSN: 1530-6984            Impact factor:   11.189


  16 in total

1.  Metal halide perovskite light emitters.

Authors:  Young-Hoon Kim; Himchan Cho; Tae-Woo Lee
Journal:  Proc Natl Acad Sci U S A       Date:  2016-09-27       Impact factor: 11.205

2.  Local Versus Long-Range Diffusion Effects of Photoexcited States on Radiative Recombination in Organic-Inorganic Lead Halide Perovskites.

Authors:  Milan Vrućinić; Clemens Matthiesen; Aditya Sadhanala; Giorgio Divitini; Stefania Cacovich; Sian E Dutton; Caterina Ducati; Mete Atatüre; Henry Snaith; Richard H Friend; Henning Sirringhaus; Felix Deschler
Journal:  Adv Sci (Weinh)       Date:  2015-07-14       Impact factor: 16.806

3.  Fabrication of Semiconducting Methylammonium Lead Halide Perovskite Particles by Spray Technology.

Authors:  Mohammad-Reza Ahmadian-Yazdi; Morteza Eslamian
Journal:  Nanoscale Res Lett       Date:  2018-01-10       Impact factor: 4.703

4.  Dismantling the "Red Wall" of Colloidal Perovskites: Highly Luminescent Formamidinium and Formamidinium-Cesium Lead Iodide Nanocrystals.

Authors:  Loredana Protesescu; Sergii Yakunin; Sudhir Kumar; Janine Bär; Federica Bertolotti; Norberto Masciocchi; Antonietta Guagliardi; Matthias Grotevent; Ivan Shorubalko; Maryna I Bodnarchuk; Chih-Jen Shih; Maksym V Kovalenko
Journal:  ACS Nano       Date:  2017-03-03       Impact factor: 15.881

5.  A Promising Beginning for Perovskite Nanocrystals: A Nano Letters Virtual Issue.

Authors:  Sarah Brittman; Jingshan Luo
Journal:  Nano Lett       Date:  2018-05-09       Impact factor: 11.189

6.  Environmental Effects on the Photophysics of Organic-Inorganic Halide Perovskites.

Authors:  Juan F Galisteo-López; M Anaya; M E Calvo; H Míguez
Journal:  J Phys Chem Lett       Date:  2015-06-01       Impact factor: 6.475

7.  Photoluminescence Blinking of Single-Crystal Methylammonium Lead Iodide Perovskite Nanorods Induced by Surface Traps.

Authors:  Haifeng Yuan; Elke Debroye; Giorgio Caliandro; Kris P F Janssen; Jordi van Loon; Christine E A Kirschhock; Johan A Martens; Johan Hofkens; Maarten B J Roeffaers
Journal:  ACS Omega       Date:  2016-07-26

8.  Degradation of Methylammonium Lead Iodide Perovskite Structures through Light and Electron Beam Driven Ion Migration.

Authors:  Haifeng Yuan; Elke Debroye; Kris Janssen; Hiroyuki Naiki; Christian Steuwe; Gang Lu; Michèle Moris; Emanuele Orgiu; Hiroshi Uji-I; Frans De Schryver; Paolo Samorì; Johan Hofkens; Maarten Roeffaers
Journal:  J Phys Chem Lett       Date:  2016-01-26       Impact factor: 6.475

9.  Harnessing Defect-Tolerance at the Nanoscale: Highly Luminescent Lead Halide Perovskite Nanocrystals in Mesoporous Silica Matrixes.

Authors:  Dmitry N Dirin; Loredana Protesescu; David Trummer; Ilia V Kochetygov; Sergii Yakunin; Frank Krumeich; Nicholas P Stadie; Maksym V Kovalenko
Journal:  Nano Lett       Date:  2016-08-25       Impact factor: 11.189

10.  Exploration of Near-Infrared-Emissive Colloidal Multinary Lead Halide Perovskite Nanocrystals Using an Automated Microfluidic Platform.

Authors:  Ioannis Lignos; Viktoriia Morad; Yevhen Shynkarenko; Caterina Bernasconi; Richard M Maceiczyk; Loredana Protesescu; Federica Bertolotti; Sudhir Kumar; Stefan T Ochsenbein; Norberto Masciocchi; Antonietta Guagliardi; Chih-Jen Shih; Maryna I Bodnarchuk; Andrew J deMello; Maksym V Kovalenko
Journal:  ACS Nano       Date:  2018-05-22       Impact factor: 15.881

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