Literature DB >> 25541780

Structural relaxation is a scale-free process.

Anaël Lemaître1.   

Abstract

We show that in deeply supercooled liquids, structural relaxation proceeds via the accumulation of Eshelby events, i.e. local rearrangements that create long-ranged and anisotropic stresses in the surrounding medium. Such events must be characterized using tensorial observables and we construct an analytical framework to probe their correlations using local stress data. By analyzing numerical simulations, we then demonstrate that events are power-law correlated in space, with a time-dependent amplitude which peaks at the alpha relaxation time τ(α). This effect, which becomes stronger near the glass transition, results from the increasingly important role of local stress fluctuations in facilitating relaxation events. Our finding precludes the existence of any length scale beyond which the relaxation process decorrelates.

Year:  2014        PMID: 25541780     DOI: 10.1103/PhysRevLett.113.245702

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  4 in total

1.  The kinetic fragility of liquids as manifestation of the elastic softening.

Authors:  F Puosi; D Leporini
Journal:  Eur Phys J E Soft Matter       Date:  2015-08-13       Impact factor: 1.890

2.  Amorphous solids: Rayleigh scattering revisited.

Authors:  Jeppe C Dyre
Journal:  Nat Mater       Date:  2016-08-29       Impact factor: 43.841

3.  Anomalous phonon scattering and elastic correlations in amorphous solids.

Authors:  Simon Gelin; Hajime Tanaka; Anaël Lemaître
Journal:  Nat Mater       Date:  2016-08-29       Impact factor: 43.841

4.  Common mechanism of thermodynamic and mechanical origin for ageing and crystallization of glasses.

Authors:  Taiki Yanagishima; John Russo; Hajime Tanaka
Journal:  Nat Commun       Date:  2017-06-29       Impact factor: 14.919

  4 in total

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