Literature DB >> 25406326

Force distribution affects vibrational properties in hard-sphere glasses.

Eric DeGiuli1, Edan Lerner2, Carolina Brito3, Matthieu Wyart4.   

Abstract

We theoretically and numerically study the elastic properties of hard-sphere glasses and provide a real-space description of their mechanical stability. In contrast to repulsive particles at zero temperature, we argue that the presence of certain pairs of particles interacting with a small force f soften elastic properties. This softening affects the exponents characterizing elasticity at high pressure, leading to experimentally testable predictions. Denoting P(f) ~ f(θ(e)), the force distribution of such pairs and ϕ(c) the packing fraction at which pressure diverges, we predict that (i) the density of states has a low-frequency peak at a scale ω*, rising up to it as D(ω) ~ ω(2+a), and decaying above ω* as D(ω) ~ ω(-a) where a = (1 - θ(e))/(3 + θ(e)) and ω is the frequency, (ii) shear modulus and mean-squared displacement are inversely proportional with ⟨δR²⟩ ~ 1/μ ~ (ϕ(c) - ϕ)(κ), where κ = 2 - 2/(3 + θ(e)), and (iii) continuum elasticity breaks down on a scale ℓ(c) ~ 1/√(δz) ~ (ϕ(c) - ϕ)(-b), where b = (1 + θ(e))/(6 + 2θ(e)) and δz = z - 2d, where z is the coordination and d the spatial dimension. We numerically test (i) and provide data supporting that θ(e) ≈ 0.41 in our bidisperse system, independently of system preparation in two and three dimensions, leading to κ ≈ 1.41, a ≈ 0.17, and b ≈ 0.21. Our results for the mean-square displacement are consistent with a recent exact replica computation for d = ∞, whereas some observations differ, as rationalized by the present approach.

Keywords:  boson peak; colloids; glass transition; jamming; marginal stability

Year:  2014        PMID: 25406326      PMCID: PMC4260553          DOI: 10.1073/pnas.1415298111

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  23 in total

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Authors:  Patrick Charbonneau; Eric I Corwin; Giorgio Parisi; Francesco Zamponi
Journal:  Phys Rev Lett       Date:  2012-11-13       Impact factor: 9.161

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Authors:  Matthieu Wyart
Journal:  Phys Rev Lett       Date:  2012-09-18       Impact factor: 9.161

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Authors:  Atsushi Ikeda; Ludovic Berthier; Giulio Biroli
Journal:  J Chem Phys       Date:  2013-03-28       Impact factor: 3.488

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Authors:  Eric DeGiuli; Adrien Laversanne-Finot; Gustavo Düring; Edan Lerner; Matthieu Wyart
Journal:  Soft Matter       Date:  2014-08-14       Impact factor: 3.679

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  7 in total

1.  Universality of jamming of nonspherical particles.

Authors:  Carolina Brito; Harukuni Ikeda; Pierfrancesco Urbani; Matthieu Wyart; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2018-10-31       Impact factor: 11.205

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Authors:  Luca Angelani; Matteo Paoluzzi; Giorgio Parisi; Giancarlo Ruocco
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Journal:  Proc Natl Acad Sci U S A       Date:  2022-05-24       Impact factor: 12.779

6.  Universal spectrum of normal modes in low-temperature glasses.

Authors:  Silvio Franz; Giorgio Parisi; Pierfrancesco Urbani; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2015-11-11       Impact factor: 11.205

7.  Exploring the complex free-energy landscape of the simplest glass by rheology.

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Journal:  Nat Commun       Date:  2017-04-11       Impact factor: 14.919

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