Literature DB >> 25388861

ω-Turn: a novel β-turn mimic in globular proteins stabilized by main-chain to side-chain C−H···O interaction.

Jesmita Dhar1, Pinak Chakrabarti, Harpreet Saini, Gajendra Pal Singh Raghava, Raghuvansh Kishore.   

Abstract

Mimicry of structural motifs is a common feature in proteins. The 10-membered hydrogen-bonded ring involving the main-chain C − O in a β-turn can be formed using a side-chain carbonyl group leading to Asx-turn. We show that the N − H component of n class="Chemical">hydrogen bond can be replaced by a C(γ) -H group in the side chain, culminating in a nonconventional C − H···O interaction. Because of its shape this β-turn mimic is designated as ω-turn, which is found to occur ∼ three times per 100 residues. Three residues (i to i + 2) constitute the turn with the C − H···O interaction occurring between the terminal residues, constraining the torsion angles ϕi + 1, ψi + 1, ϕi + 2 and χ'1(i + 2) (using the interacting C(γ) atom). Based on these angles there are two types of ω-turns, each of which can be further divided into two groups. C(β) -branched side-chains, and Met and Gln have high propensities to occur at i + 2; for the last two residues the carbonyl oxygen may participate in an additional interaction involving the S and amino group, respectively. With Cys occupying the i + 1 position, such turns are found in the metal-binding sites. N-linked glycosylation occurs at the consensus pattern Asn-Xaa-Ser/Thr; with Thr at i + 2, the sequence can adopt the secondary structure of a ω-turn, which may be the recognition site for protein modification. Location between two β-strands is the most common occurrence in protein tertiary structure, and being generally exposed ω-turn may constitute the antigenic determinant site. It is a stable scaffold and may be used in protein engineering and peptide design.
© 2014 Wiley Periodicals, Inc.

Entities:  

Keywords:  CH···O interaction; N-linked glycosylation; weak interactions in protein structures; β-turn mimicry; ω-turn

Mesh:

Substances:

Year:  2014        PMID: 25388861     DOI: 10.1002/prot.24720

Source DB:  PubMed          Journal:  Proteins        ISSN: 0887-3585


  2 in total

1.  A novel secondary structure based on fused five-membered rings motif.

Authors:  Jesmita Dhar; Raghuvansh Kishore; Pinak Chakrabarti
Journal:  Sci Rep       Date:  2016-08-11       Impact factor: 4.379

2.  The susceptibility of disulfide bonds towards radiation damage may be explained by S⋯O interactions.

Authors:  Rajasri Bhattacharyya; Jesmita Dhar; Shubhra Ghosh Dastidar; Pinak Chakrabarti; Manfred S Weiss
Journal:  IUCrJ       Date:  2020-07-24       Impact factor: 4.769

  2 in total

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