Literature DB >> 25313063

Recent distribution of lead in the Indian Ocean reflects the impact of regional emissions.

Yolanda Echegoyen1, Edward A Boyle2, Jong-Mi Lee3, Toshitaka Gamo4, Hajime Obata4, Kazuhiro Norisuye5.   

Abstract

Humans have injected lead (Pb) massively into the earth surface environment in a temporally and spatially evolving pattern. A significant fraction is transported by the atmosphere into the surface ocean where we can observe its transport by ocean currents and sinking particles. This study of the Indian Ocean documents high Pb concentrations in the northern and tropical surface waters and extremely low Pb levels in the deep water. North of 20°S, dissolved Pb concentrations decrease from 42 to 82 pmol/kg in surface waters to 1.5-3.3 pmol/kg in deep waters. South of 20°S, surface water Pb concentrations decrease from 21 pmol/kg at 31°S to 7 pmol/kg at 62°S. This surface Pb concentration gradient reflects a southward decrease in anthropogenic Pb emissions. The upper waters of the north and central Indian Ocean have high Pb concentrations resulting from recent regional rapid industrialization and a late phase-out of leaded gasoline, and these concentrations are now higher than currently seen in the central North Pacific and North Atlantic oceans. The Antarctic sector of the Indian Ocean shows very low concentrations due to limited regional anthropogenic Pb emissions, high scavenging rates, and rapid vertical mixing, but Pb still occurs at higher levels than would have existed centuries ago. Penetration of Pb into the northern and central Indian Ocean thermocline waters is minimized by limited ventilation. Pb concentrations in the deep Indian Ocean are comparable to the other oceans at the same latitude, and deep waters of the central Indian Ocean match the lowest observed oceanic Pb concentrations.

Entities:  

Keywords:  GEOTRACES; Indian Ocean; Pb content; anthropogenic emissions; lead

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Year:  2014        PMID: 25313063      PMCID: PMC4217456          DOI: 10.1073/pnas.1417370111

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  2 in total

1.  Asian industrial lead inputs to the North Pacific evidenced by lead concentrations and isotopic compositions in surface waters and aerosols.

Authors:  Céline Gallon; Mara A Ranville; Christopher H Conaway; William M Landing; Clifton S Buck; Peter L Morton; A Russell Flegal
Journal:  Environ Sci Technol       Date:  2011-11-08       Impact factor: 9.028

2.  Analysis of trace metals (Cu, Cd, Pb, and Fe) in seawater using single batch nitrilotriacetate resin extraction and isotope dilution inductively coupled plasma mass spectrometry.

Authors:  Jong-Mi Lee; Edward A Boyle; Yolanda Echegoyen-Sanz; Jessica N Fitzsimmons; Ruifeng Zhang; Richard A Kayser
Journal:  Anal Chim Acta       Date:  2010-12-10       Impact factor: 6.558

  2 in total
  1 in total

1.  Anthropogenic Asian aerosols provide Fe to the North Pacific Ocean.

Authors:  Paulina Pinedo-González; Nicholas J Hawco; Randelle M Bundy; E Virginia Armbrust; Michael J Follows; B B Cael; Angelicque E White; Sara Ferrón; David M Karl; Seth G John
Journal:  Proc Natl Acad Sci U S A       Date:  2020-10-22       Impact factor: 11.205

  1 in total

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