Literature DB >> 24920053

Catalytic biorefining of plant biomass to non-pyrolytic lignin bio-oil and carbohydrates through hydrogen transfer reactions.

Paola Ferrini1, Roberto Rinaldi.   

Abstract

Through catalytic hydrogen transfer reactions, a new biorefining method results in the isolation of depolymerized lignin--a non-pyrolytic lignin bio-oil--in addition to pulps that are amenable to enzymatic hydrolysis. Compared with organosolv lignin, the lignin bio-oil is highly susceptible to further hydrodeoxygenation under low-severity conditions and therefore establishes a unique platform for lignin valorization by heterogeneous catalysis. Overall, the potential of a catalytic biorefining method designed from the perspective of lignin utilization is reported.
© 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Entities:  

Keywords:  biorefinery; catalytic hydrogen transfer; cellulose; enzymatic hydrolysis; lignin

Mesh：

Substances：

Year:  2014        PMID： 24920053     DOI： 10.1002/anie.201403747

Source DB:  PubMed          Journal:  Angew Chem Int Ed Engl        ISSN： 1433-7851            Impact factor:   15.336


  20 in total

1.  Bright Side of Lignin Depolymerization: Toward New Platform Chemicals.

Authors:  Zhuohua Sun; Bálint Fridrich; Alessandra de Santi; Saravanakumar Elangovan; Katalin Barta
Journal:  Chem Rev       Date:  2018-01-16       Impact factor: 60.622

Review 2.  Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis.

Authors:  Roberto Rinaldi; Robin Jastrzebski; Matthew T Clough; John Ralph; Marco Kennema; Pieter C A Bruijnincx; Bert M Weckhuysen
Journal:  Angew Chem Int Ed Engl       Date:  2016-06-17       Impact factor: 15.336

Review 3.  Homogeneous Catalysis for Sustainable Energy: Hydrogen and Methanol Economies, Fuels from Biomass, and Related Topics.

Authors:  Amit Kumar; Prosenjit Daw; David Milstein
Journal:  Chem Rev       Date:  2021-11-02       Impact factor: 60.622

4.  Selective production of arenes via direct lignin upgrading over a niobium-based catalyst.

Authors:  Yi Shao; Qineng Xia; Lin Dong; Xiaohui Liu; Xue Han; Stewart F Parker; Yongqiang Cheng; Luke L Daemen; Anibal J Ramirez-Cuesta; Sihai Yang; Yanqin Wang
Journal:  Nat Commun       Date:  2017-07-24       Impact factor: 14.919

5.  Lignin Hydrogenolysis: Improving Lignin Disassembly through Formaldehyde Stabilization.

Authors:  Markus D Kärkäs
Journal:  ChemSusChem       Date:  2017-05-05       Impact factor: 8.928

Review 6.  Lignocellulose Liquefaction to Biocrude: A Tutorial Review.

Authors:  Jean-Paul Lange
Journal:  ChemSusChem       Date:  2018-03-13       Impact factor: 8.928

7.  From Tree to Tape: Direct Synthesis of Pressure Sensitive Adhesives from Depolymerized Raw Lignocellulosic Biomass.

Authors:  Shu Wang; Li Shuai; Basudeb Saha; Dionisios G Vlachos; Thomas H Epps
Journal:  ACS Cent Sci       Date:  2018-05-15       Impact factor: 14.553

8.  Reductive catalytic fractionation of pine wood: elucidating and quantifying the molecular structures in the lignin oil.

Authors:  K Van Aelst; E Van Sinay; T Vangeel; E Cooreman; G Van den Bossche; T Renders; J Van Aelst; S Van den Bosch; B F Sels
Journal:  Chem Sci       Date:  2020-09-26       Impact factor: 9.825

9.  Highly selective hydrogenation of arenes using nanostructured ruthenium catalysts modified with a carbon-nitrogen matrix.

Authors:  Xinjiang Cui; Annette-Enrica Surkus; Kathrin Junge; Christoph Topf; Jörg Radnik; Carsten Kreyenschulte; Matthias Beller
Journal:  Nat Commun       Date:  2016-04-26       Impact factor: 14.919

10.  Tandem Catalytic Depolymerization of Lignin by Water-Tolerant Lewis Acids and Rhodium Complexes.

Authors:  Robin Jastrzebski; Sandra Constant; Christopher S Lancefield; Nicholas J Westwood; Bert M Weckhuysen; Pieter C A Bruijnincx
Journal:  ChemSusChem       Date:  2016-07-21       Impact factor: 8.928
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