Literature DB >> 24815658

Two-level systems and boson peak remain stable in 110-million-year-old amber glass.

Tomás Pérez-Castañeda1, Rafael J Jiménez-Riobóo2, Miguel A Ramos1.   

Abstract

The two most prominent and ubiquitous features of glasses at low temperatures, namely the presence of tunneling two-level systems and the so-called boson peak in the reduced vibrational density of states, are shown to persist essentially unchanged in highly stabilized glasses, contrary to what was usually envisaged. Specifically, we have measured the specific heat of 110 million-year-old amber samples from El Soplao (Spain), both at very low temperatures and around the glass transition Tg. In particular, the amount of two-level systems, assessed at the lowest temperatures, was surprisingly found to be exactly the same for the pristine hyperaged amber as for the, subsequently, partially and fully rejuvenated samples.

Entities:  

Year:  2014        PMID: 24815658     DOI: 10.1103/PhysRevLett.112.165901

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  8 in total

1.  Vapor-deposited glasses provide clearer view of two-level systems.

Authors:  M D Ediger
Journal:  Proc Natl Acad Sci U S A       Date:  2014-07-22       Impact factor: 11.205

2.  Suppression of tunneling two-level systems in ultrastable glasses of indomethacin.

Authors:  Tomás Pérez-Castañeda; Cristian Rodríguez-Tinoco; Javier Rodríguez-Viejo; Miguel A Ramos
Journal:  Proc Natl Acad Sci U S A       Date:  2014-07-07       Impact factor: 11.205

3.  Relaxation dynamics of glasses along a wide stability and temperature range.

Authors:  C Rodríguez-Tinoco; J Ràfols-Ribé; M González-Silveira; J Rodríguez-Viejo
Journal:  Sci Rep       Date:  2016-10-21       Impact factor: 4.379

4.  Emergence of a substrate-temperature-dependent dielectric process in a prototypical vapor deposited hole-transport glass.

Authors:  Cristian Rodríguez-Tinoco; Marzena Rams-Baron; Javier Rodríguez-Viejo; Marian Paluch
Journal:  Sci Rep       Date:  2018-01-22       Impact factor: 4.379

5.  Ultrastable metallic glass by room temperature aging.

Authors:  Yong Zhao; Baoshuang Shang; Bo Zhang; Xing Tong; Haibo Ke; Haiyang Bai; Wei-Hua Wang
Journal:  Sci Adv       Date:  2022-08-17       Impact factor: 14.957

6.  Low-temperature excess heat capacity in fresnoite glass and crystal.

Authors:  Kensaku Nakamura; Yoshihiro Takahashi; Takumi Fujiwara
Journal:  Sci Rep       Date:  2014-10-06       Impact factor: 4.379

7.  Ultrastable glasses portray similar behaviour to ordinary glasses at high pressure.

Authors:  C Rodríguez-Tinoco; M González-Silveira; M Barrio; P Lloveras; J Ll Tamarit; J-L Garden; J Rodríguez-Viejo
Journal:  Sci Rep       Date:  2016-10-03       Impact factor: 4.379

8.  Boson peak, elasticity, and glass transition temperature in polymer glasses: Effects of the rigidity of chain bending.

Authors:  Naoya Tomoshige; Hideyuki Mizuno; Tatsuya Mori; Kang Kim; Nobuyuki Matubayasi
Journal:  Sci Rep       Date:  2019-12-20       Impact factor: 4.379

  8 in total

北京卡尤迪生物科技股份有限公司 © 2022-2023.