Literature DB >> 24226888

Stabilizing the magnetic moment of single holmium atoms by symmetry.

Toshio Miyamachi1, Tobias Schuh, Tobias Märkl, Christopher Bresch, Timofey Balashov, Alexander Stöhr, Christian Karlewski, Stephan André, Michael Marthaler, Martin Hoffmann, Matthias Geilhufe, Sergey Ostanin, Wolfram Hergert, Ingrid Mertig, Gerd Schön, Arthur Ernst, Wulf Wulfhekel.   

Abstract

Single magnetic atoms, and assemblies of such atoms, on non-magnetic surfaces have recently attracted attention owing to their potential use in high-density magnetic data storage and as a platform for quantum computing. A fundamental problem resulting from their quantum mechanical nature is that the localized magnetic moments of these atoms are easily destabilized by interactions with electrons, nuclear spins and lattice vibrations of the substrate. Even when large magnetic fields are applied to stabilize the magnetic moment, the observed lifetimes remain rather short (less than a microsecond). Several routes for stabilizing the magnetic moment against fluctuations have been suggested, such as using thin insulating layers between the magnetic atom and the substrate to suppress the interactions with the substrate's conduction electrons, or coupling several magnetic moments together to reduce their quantum mechanical fluctuations. Here we show that the magnetic moments of single holmium atoms on a highly conductive metallic substrate can reach lifetimes of the order of minutes. The necessary decoupling from the thermal bath of electrons, nuclear spins and lattice vibrations is achieved by a remarkable combination of several symmetries intrinsic to the system: time reversal symmetry, the internal symmetries of the total angular momentum and the point symmetry of the local environment of the magnetic atom.

Entities:  

Year:  2013        PMID: 24226888     DOI: 10.1038/nature12759

Source DB:  PubMed          Journal:  Nature        ISSN: 0028-0836            Impact factor:   49.962


  16 in total

1.  The remarkable difference between surface and step atoms in the magnetic anisotropy of two-dimensional nanostructures.

Authors:  S Rusponi; T Cren; N Weiss; M Epple; P Buluschek; L Claude; H Brune
Journal:  Nat Mater       Date:  2003-08       Impact factor: 43.841

2.  Calculated crystal-field parameters of SmCo5.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1992-12-01

3.  Single-atom spin-flip spectroscopy.

Authors:  A J Heinrich; J A Gupta; C P Lutz; D M Eigler
Journal:  Science       Date:  2004-09-09       Impact factor: 47.728

4.  Bistability in atomic-scale antiferromagnets.

Authors:  Sebastian Loth; Susanne Baumann; Christopher P Lutz; D M Eigler; Andreas J Heinrich
Journal:  Science       Date:  2012-01-13       Impact factor: 47.728

5.  Measurement of fast electron spin relaxation times with atomic resolution.

Authors:  Sebastian Loth; Markus Etzkorn; Christopher P Lutz; D M Eigler; Andreas J Heinrich
Journal:  Science       Date:  2010-09-24       Impact factor: 47.728

6.  Large magnetic anisotropy of a single atomic spin embedded in a surface molecular network.

Authors:  Cyrus F Hirjibehedin; Chiung-Yuan Lin; Alexander F Otte; Markus Ternes; Christopher P Lutz; Barbara A Jones; Andreas J Heinrich
Journal:  Science       Date:  2007-08-31       Impact factor: 47.728

7.  Ab-initio simulations of materials using VASP: Density-functional theory and beyond.

Authors:  Jürgen Hafner
Journal:  J Comput Chem       Date:  2008-10       Impact factor: 3.376

8.  Itinerant nature of atom-magnetization excitation by tunneling electrons.

Authors:  A A Khajetoorians; S Lounis; B Chilian; A T Costa; L Zhou; D L Mills; J Wiebe; R Wiesendanger
Journal:  Phys Rev Lett       Date:  2011-01-20       Impact factor: 9.161

9.  Magnetic excitations of rare earth atoms and clusters on metallic surfaces.

Authors:  Tobias Schuh; Toshio Miyamachi; Stefan Gerstl; Matthias Geilhufe; Martin Hoffmann; Sergey Ostanin; Wolfram Hergert; Arthur Ernst; Wulf Wulfhekel
Journal:  Nano Lett       Date:  2012-08-22       Impact factor: 11.189

10.  A compact sub-Kelvin ultrahigh vacuum scanning tunneling microscope with high energy resolution and high stability.

Authors:  L Zhang; T Miyamachi; T Tomanić; R Dehm; W Wulfhekel
Journal:  Rev Sci Instrum       Date:  2011-10       Impact factor: 1.523

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  16 in total

1.  Magnetic properties: the exchange changes everything.

Authors:  Wulf Wulfhekel
Journal:  Nat Nanotechnol       Date:  2014-01       Impact factor: 39.213

2.  Quantum physics: The right ambience for a single spin.

Authors:  Michael E Flatté
Journal:  Nature       Date:  2013-11-14       Impact factor: 49.962

3.  Spin waves: close-up on spin dynamics.

Authors:  Stanislas Rohart; Guillemin Rodary
Journal:  Nat Mater       Date:  2014-07-06       Impact factor: 43.841

4.  Meta-Atom Behavior in Clusters Revealing Large Spin Ground States.

Authors:  Raúl Hernández Sánchez; Theodore A Betley
Journal:  J Am Chem Soc       Date:  2015-10-21       Impact factor: 15.419

5.  Enhanced magnetic anisotropies of single transition-metal adatoms on a defective MoS2 monolayer.

Authors:  W T Cong; Z Tang; X G Zhao; J H Chu
Journal:  Sci Rep       Date:  2015-03-23       Impact factor: 4.379

6.  Engineering atomic-scale magnetic fields by dysprosium single atom magnets.

Authors:  A Singha; P Willke; T Bilgeri; X Zhang; H Brune; F Donati; A J Heinrich; T Choi
Journal:  Nat Commun       Date:  2021-07-07       Impact factor: 14.919

7.  Integrated information storage and transfer with a coherent magnetic device.

Authors:  Ning Jia; Leonardo Banchi; Abolfazl Bayat; Guangjiong Dong; Sougato Bose
Journal:  Sci Rep       Date:  2015-09-08       Impact factor: 4.379

8.  Antiferromagnetic Spin Coupling between Rare Earth Adatoms and Iron Islands Probed by Spin-Polarized Tunneling.

Authors:  David Coffey; José Luis Diez-Ferrer; David Serrate; Miguel Ciria; César de la Fuente; José Ignacio Arnaudas
Journal:  Sci Rep       Date:  2015-09-03       Impact factor: 4.379

9.  Quantum engineering of spin and anisotropy in magnetic molecular junctions.

Authors:  Peter Jacobson; Tobias Herden; Matthias Muenks; Gennadii Laskin; Oleg Brovko; Valeri Stepanyuk; Markus Ternes; Klaus Kern
Journal:  Nat Commun       Date:  2015-10-12       Impact factor: 14.919

10.  Dynamically Tuning the Up-conversion Luminescence of Er(3+)/Yb(3+) Co-doped Sodium Niobate Nano-crystals through Magnetic Field.

Authors:  Quanlan Xiao; Yuanhao Zhang; Han Zhang; Guoping Dong; Junbo Han; Jianrong Qiu
Journal:  Sci Rep       Date:  2016-08-09       Impact factor: 4.379

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