Literature DB >> 24182044

Dimensional dependence of the Stokes-Einstein relation and its violation.

Benoit Charbonneau1, Patrick Charbonneau, Yuliang Jin, Giorgio Parisi, Francesco Zamponi.   

Abstract

We generalize to higher spatial dimensions the Stokes-Einstein relation (SER) as well as the leading correction to diffusivity in finite systems with periodic boundary conditions, and validate these results with numerical simulations. We then investigate the evolution of the high-density SER violation with dimension in simple hard sphere glass formers. The analysis suggests that this SER violation disappears around dimension d(u) = 8, above which it is not observed. The critical exponent associated with the violation appears to evolve linearly in 8 - d, below d = 8, as predicted by Biroli and Bouchaud [J. Phys.: Condens. Matter 19, 205101 (2007)], but the linear coefficient is not consistent with the prediction. The SER violation with d establishes a new benchmark for theory, and its complete description remains an open problem.

Entities:  

Year:  2013        PMID: 24182044     DOI: 10.1063/1.4825177

Source DB:  PubMed          Journal:  J Chem Phys        ISSN: 0021-9606            Impact factor:   3.488


  3 in total

1.  Power law relationship between diffusion coefficients in multi-component glass forming liquids.

Authors:  Anshul D S Parmar; Shiladitya Sengupta; Srikanth Sastry
Journal:  Eur Phys J E Soft Matter       Date:  2018-08-08       Impact factor: 1.890

2.  Calorimetric glass transition in a mean-field theory approach.

Authors:  Manuel Sebastian Mariani; Giorgio Parisi; Corrado Rainone
Journal:  Proc Natl Acad Sci U S A       Date:  2015-02-09       Impact factor: 11.205

3.  Hopping and the Stokes-Einstein relation breakdown in simple glass formers.

Authors:  Patrick Charbonneau; Yuliang Jin; Giorgio Parisi; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2014-10-06       Impact factor: 11.205

  3 in total

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