| Literature DB >> 24182020 |
Leonardo A Pachón1, Paul Brumer.
Abstract
The ability of an environment to assist in one-photon phase control relies upon entanglement between the system and bath and on the breaking of the time reversal symmetry. Here, one-photon phase control is examined analytically and numerically in a model system, allowing an analysis of the relative strength of these contributions. Further, the significant role of non-Markovian dynamics and of moderate system-bath coupling in enhancing one-photon phase control is demonstrated, and an explicit role for quantum mechanics is noted in the existence of initial non-zero stationary coherences. Finally, desirable conditions are shown to be required to observe such environmentally assisted control, since the system will naturally equilibrate with its environment at longer times, ultimately resulting in the loss of phase control.Year: 2013 PMID: 24182020 DOI: 10.1063/1.4825358
Source DB: PubMed Journal: J Chem Phys ISSN: 0021-9606 Impact factor: 3.488