Literature DB >> 23742467

Measurement of the Soret coefficients for a ternary hydrocarbon mixture in low gravity environment.

Amirhossein Ahadi1, S Van Varenbergh, M Ziad Saghir.   

Abstract

While the Soret coefficients of binary mixtures have been widely measured in the past, here we report the first measurement of the Soret coefficient of a ternary mixture in a low gravity environment on board the International Space Station. The sample was contained in a 10 mm × 10 mm × 5 mm (w, l, h) cell and was monitored by means of a Mach-Zehnder interferometer at two wavelengths. The analyzed sample was a mixture of tetrahydronaphthalene, isobutylbenzene, and dodecane at the weight fraction of 0.1∕0.8∕0.1. While the lateral walls of the cell did not possess complete thermal isolation, the separation of the components in the central region of the cavity was comparable to purely diffusive behavior. The same experimental parameters have been monitored in Run7 and Run12 of the Selectable Optical Diagnostics Instrument-Diffusion and Soret Coefficient experiment in order to verify the accuracy of the setup. The similarity of the results demonstrates the repeatability of thermodiffusion experiments in a microgravity environment. There was nearly equal separation of the tetrahydronaphthalene and isobutylbenzene components in opposite directions, while dodecane experienced a weak separation in the same direction as isobutylbenzene. Finally, Fourier image processing and calculations of the transient separation of the components were used to analyze the heat transfer in the system and to measure the Soret coefficients for this ternary mixture. The successful measurements shown in this work can serve as the standard for ground experiments and for numerical modeling of hydrocarbon mixtures.

Entities:  

Year:  2013        PMID: 23742467     DOI: 10.1063/1.4802984

Source DB:  PubMed          Journal:  J Chem Phys        ISSN: 0021-9606            Impact factor:   3.488


  6 in total

1.  Benchmark values for the Soret, thermodiffusion and molecular diffusion coefficients of the ternary mixture tetralin+isobutylbenzene+n-dodecane with 0.8-0.1-0.1 mass fraction.

Authors:  M M Bou-Ali; A Ahadi; D Alonso de Mezquia; Q Galand; M Gebhardt; O Khlybov; W Köhler; M Larrañaga; J C Legros; T Lyubimova; A Mialdun; I Ryzhkov; M Z Saghir; V Shevtsova; S Van Vaerenbergh
Journal:  Eur Phys J E Soft Matter       Date:  2015-04-28       Impact factor: 1.890

2.  Preliminary analysis of Diffusion Coefficient Measurements in ternary mIXtures 4 (DCMIX4) experiment on board the International Space Station.

Authors:  A Mialdun; H Bataller; M M Bou-Ali; M Braibanti; F Croccolo; A Errarte; J M Ezquerro; J J Fernández; Yu Gaponenko; L García-Fernández; J Rodríguez; V Shevtsova
Journal:  Eur Phys J E Soft Matter       Date:  2019-07-11       Impact factor: 1.890

3.  Non-equilibrium fluctuations induced by the Soret effect in a ternary mixture.

Authors:  José M Ortiz de Zárate; Cédric Giraudet; Henri Bataller; Fabrizio Croccolo
Journal:  Eur Phys J E Soft Matter       Date:  2014-08-28       Impact factor: 1.890

4.  Contribution to the benchmark for ternary mixtures: Measurement of diffusion and Soret coefficients of ternary system tetrahydronaphtalene-isobutylbenzene-n-dodecane with mass fractions 80-10-10 at 25 °C.

Authors:  Quentin Galand; Stéfan Van Vaerenbergh
Journal:  Eur Phys J E Soft Matter       Date:  2015-04-27       Impact factor: 1.890

5.  Contribution to the benchmark for ternary mixtures: Transient analysis in microgravity conditions.

Authors:  Amirhossein Ahadi; M Ziad Saghir
Journal:  Eur Phys J E Soft Matter       Date:  2015-04-27       Impact factor: 1.890

6.  Differential dynamic microscopy of bidisperse colloidal suspensions.

Authors:  Mohammad S Safari; Ryan Poling-Skutvik; Peter G Vekilov; Jacinta C Conrad
Journal:  NPJ Microgravity       Date:  2017-08-30       Impact factor: 4.415

  6 in total

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