Coherent control of light scattering from nanostructured materials by second-harmonic generation.

We introduce an active, all-optical method for controlling the intensity and directionality of light scattering from single nanostructures. The method is based on the coherent interplay between linear light scattering and second-harmonic generation. The intensity and directionality of scattered light can be controlled by the phase delay and the relative angle between excitation beams. We discuss the principle of this coherent control technique and perform numerical model calculations.