Literature DB >> 23660772

Methotrexate binds to recombinant thiopurine S-methyltransferase and inhibits enzyme activity after high-dose infusions in childhood leukaemia.

Patricia Wennerstrand1, Lars-Göran Mårtensson, Stefan Söderhäll, Anna Zimdahl, Malin Lindqvist Appell.   

Abstract

PURPOSE: Important drugs in the treatment of childhood acute lymphoblastic leukaemia (ALL) are 6-mercaptopurine (6-MP) and methotrexate (MTX). Thiopurine methyltransferase (TPMT) is a polymorphic enzyme causing variability in 6-MP response and toxicity. The aim of this study was to investigate the fluctuation in TPMT enzyme activity over time and the effect of high-dose MTX infusions on TPMT enzyme activity and 6-MP metabolites in paediatric ALL patients.
METHODS: Fifty-three children with ALL treated according to the NOPHO-ALL 2000 protocol were included in the study. TPMT enzyme activity was measured at six different times starting from diagnosis until after the end of maintenance treatment. TPMT and 6-MP metabolites were measured before the initiation of high-dose MTX (HD-MTX) infusions and at 66 h post-infusion. The interaction between MTX and TPMT was investigated in vitro using recombinant TPMT protein and a leukaemic cell line.
RESULTS: Forty percent of TPMT wild-type individuals had deceptively low TPMT enzyme activity according to genotype at the time of diagnosis. TPMT activity had decreased significantly 66 h after the start of HD-MTX infusions (-9.2 %; p = 0.013). MTX bound to recombinant TPMT protein severely inhibiting TPMT enzyme activity (remaining activity 16 %).
CONCLUSIONS: Our results show that TPMT genotyping should be performed in children with ALL, since 40 % of the children in our study who carried the wild-type TPMT gene were at risk of initial underdosing of 6-MP in cases where only TPMT enzyme activity was determined. MTX inhibits the TPMT enzyme activity after HD-MTX infusions due to protein binding.

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Year:  2013        PMID: 23660772     DOI: 10.1007/s00228-013-1521-9

Source DB:  PubMed          Journal:  Eur J Clin Pharmacol        ISSN: 0031-6970            Impact factor:   2.953


  21 in total

1.  Structural basis of allele variation of human thiopurine-S-methyltransferase.

Authors:  Hong Wu; John R Horton; Kevin Battaile; Abdellah Allali-Hassani; Fernando Martin; Hong Zeng; Peter Loppnau; Masoud Vedadi; Alexey Bochkarev; Alexander N Plotnikov; Xiaodong Cheng
Journal:  Proteins       Date:  2007-04-01

2.  Mercaptopurine therapy intolerance and heterozygosity at the thiopurine S-methyltransferase gene locus.

Authors:  M V Relling; M L Hancock; G K Rivera; J T Sandlund; R C Ribeiro; E Y Krynetski; C H Pui; W E Evans
Journal:  J Natl Cancer Inst       Date:  1999-12-01       Impact factor: 13.506

3.  Gene expression and thioguanine nucleotide disposition in acute lymphoblastic leukemia after in vivo mercaptopurine treatment.

Authors:  Gianluigi Zaza; Meyling Cheok; Wenjian Yang; John C Panetta; Ching-Hon Pui; Mary V Relling; William E Evans
Journal:  Blood       Date:  2005-05-19       Impact factor: 22.113

4.  Thiopurine methyltransferase in acute lymphoblastic leukaemia: biochemical and molecular biological aspects.

Authors:  Connie Brouwer; Ronney A De Abreu; Jenneke J Keizer-Garritsen; Lambert H J Lambooy; Kai Ament; Patricia G J H ter Riet; Elisabeth R van Wering; Frans J M Trijbels; Anjo J P Veerman; Peter M Hoogerbrugge; Jos P M Bökkerink
Journal:  Eur J Cancer       Date:  2005-01-20       Impact factor: 9.162

5.  Identification of two novel sequence variants affecting thiopurine methyltransferase enzyme activity.

Authors:  Malin Lindqvist; Sofie Haglund; Sven Almer; Curt Peterson; Jan Taipalensu; Erik Hertervig; Ebbe Lyrenäs; Peter Söderkvist
Journal:  Pharmacogenetics       Date:  2004-04

6.  De novo purine synthesis inhibition and antileukemic effects of mercaptopurine alone or in combination with methotrexate in vivo.

Authors:  Thierry Dervieux; Timothy L Brenner; Yuen Y Hon; Yinmei Zhou; Michael L Hancock; John T Sandlund; Gaston K Rivera; Raul C Ribeiro; James M Boyett; Ching-Hon Pui; Mary V Relling; William E Evans
Journal:  Blood       Date:  2002-08-15       Impact factor: 22.113

7.  Mercaptopurine pharmacogenetics: monogenic inheritance of erythrocyte thiopurine methyltransferase activity.

Authors:  R M Weinshilboum; S L Sladek
Journal:  Am J Hum Genet       Date:  1980-09       Impact factor: 11.025

8.  Methylation of mercaptopurine, thioguanine, and their nucleotide metabolites by heterologously expressed human thiopurine S-methyltransferase.

Authors:  E Y Krynetski; N F Krynetskaia; Y Yanishevski; W E Evans
Journal:  Mol Pharmacol       Date:  1995-06       Impact factor: 4.436

9.  Altered mercaptopurine metabolism, toxic effects, and dosage requirement in a thiopurine methyltransferase-deficient child with acute lymphocytic leukemia.

Authors:  W E Evans; M Horner; Y Q Chu; D Kalwinsky; W M Roberts
Journal:  J Pediatr       Date:  1991-12       Impact factor: 4.406

10.  Thiopurine methyltransferase genotype-phenotype discordance and thiopurine active metabolite formation in childhood acute lymphoblastic leukaemia.

Authors:  Lynne Lennard; Cher Suzanne Cartwright; Rachel Wade; Susan M Richards; Ajay Vora
Journal:  Br J Clin Pharmacol       Date:  2013-07       Impact factor: 4.335

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  9 in total

1.  Genetic and metabolic determinants of methotrexate-induced mucositis in pediatric acute lymphoblastic leukemia.

Authors:  M A H den Hoed; E Lopez-Lopez; M L te Winkel; W Tissing; J D E de Rooij; A Gutierrez-Camino; A Garcia-Orad; E den Boer; R Pieters; S M F Pluijm; R de Jonge; M M van den Heuvel-Eibrink
Journal:  Pharmacogenomics J       Date:  2014-11-04       Impact factor: 3.550

2.  No association between relapse hazard and thiopurine methyltransferase geno- or phenotypes in non-high risk acute lymphoblastic leukemia: a NOPHO ALL2008 sub-study.

Authors:  Stine Nygaard Nielsen; Linea Natalie Toksvang; Kathrine Grell; Jacob Nersting; Jonas Abrahamsson; Bendik Lund; Jukka Kanerva; Ólafur Gísli Jónsson; Goda Vaitkeviciene; Kaie Pruunsild; Malin Lindqvist Appell; Lisa Lyngsie Hjalgrim; Kjeld Schmiegelow
Journal:  Cancer Chemother Pharmacol       Date:  2021-04-29       Impact factor: 3.333

3.  High frequency of mutant thiopurine S-methyltransferase genotypes in Mexican patients with systemic lupus erythematosus and rheumatoid arthritis.

Authors:  Mireya Ramirez-Florencio; Silvia Jiménez-Morales; Rosa Elda Barbosa-Cobos; Daniela Josabeth López-Cano; Julian Ramírez-Bello
Journal:  Clin Rheumatol       Date:  2017-12-20       Impact factor: 2.980

4.  Thiopurine S-methyltransferase testing for averting drug toxicity in patients receiving thiopurines: a systematic review.

Authors:  Lilla M Roy; Richard M Zur; Elizabeth Uleryk; Chris Carew; Shinya Ito; Wendy J Ungar
Journal:  Pharmacogenomics       Date:  2016-03-29       Impact factor: 2.533

Review 5.  Thiopurine S-methyltransferase testing for averting drug toxicity: a meta-analysis of diagnostic test accuracy.

Authors:  R M Zur; L M Roy; S Ito; J Beyene; C Carew; W J Ungar
Journal:  Pharmacogenomics J       Date:  2016-05-24       Impact factor: 3.550

6.  In Vitro Protein Stability of Two Naturally Occurring Thiopurine S-Methyltransferase Variants: Biophysical Characterization of TPMT*6 and TPMT*8.

Authors:  Patricia Wennerstrand; Annica Blissing; Lars-Göran Mårtensson
Journal:  ACS Omega       Date:  2017-08-28

Review 7.  Update on the Pathomechanism, Diagnosis, and Treatment Options for Rheumatoid Arthritis.

Authors:  Yen-Ju Lin; Martina Anzaghe; Stefan Schülke
Journal:  Cells       Date:  2020-04-03       Impact factor: 6.600

8.  Changes in intracellular folate metabolism during high-dose methotrexate and Leucovorin rescue therapy in children with acute lymphoblastic leukemia.

Authors:  Natanja Oosterom; Robert de Jonge; Desiree E C Smith; Rob Pieters; Wim J E Tissing; Marta Fiocco; Bertrand D van Zelst; Marry M van den Heuvel-Eibrink; Sandra G Heil
Journal:  PLoS One       Date:  2019-09-17       Impact factor: 3.240

Review 9.  Pharmacogenetic studies of thiopurine methyltransferase genotype-phenotype concordance and effect of methotrexate on thiopurine metabolism.

Authors:  Anna Zimdahl Kahlin; Sara Helander; Patricia Wennerstrand; Svante Vikingsson; Lars-Göran Mårtensson; Malin Lindqvist Appell
Journal:  Basic Clin Pharmacol Toxicol       Date:  2020-09-14       Impact factor: 4.080

  9 in total

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