Literature DB >> 23406134

Compressed correlation functions and fast aging dynamics in metallic glasses.

B Ruta1, G Baldi, G Monaco, Y Chushkin.   

Abstract

We present x-ray photon correlation spectroscopy measurements of the atomic dynamics in a Zr(67)Ni(33) metallic glass, well below its glass transition temperature. We find that the decay of the density fluctuations can be well described by compressed, thus faster than exponential, correlation functions which can be modeled by the well-known Kohlrausch-Williams-Watts function with a shape exponent β larger than one. This parameter is furthermore found to be independent of both waiting time and wave-vector, leading to the possibility to rescale all the correlation functions to a single master curve. The dynamics in the glassy state is additionally characterized by different aging regimes which persist in the deep glassy state. These features seem to be universal in metallic glasses and suggest a nondiffusive nature of the dynamics. This universality is supported by the possibility of describing the fast increase of the structural relaxation time with waiting time using a unique model function, independently of the microscopic details of the system.

Year:  2013        PMID: 23406134     DOI: 10.1063/1.4790131

Source DB:  PubMed          Journal:  J Chem Phys        ISSN: 0021-9606            Impact factor:   3.488


  5 in total

1.  Avalanches mediate crystallization in a hard-sphere glass.

Authors:  Eduardo Sanz; Chantal Valeriani; Emanuela Zaccarelli; Wilson C K Poon; Michael E Cates; Peter N Pusey
Journal:  Proc Natl Acad Sci U S A       Date:  2013-12-04       Impact factor: 11.205

2.  Unveiling the structural arrangements responsible for the atomic dynamics in metallic glasses during physical aging.

Authors:  V M Giordano; B Ruta
Journal:  Nat Commun       Date:  2016-01-20       Impact factor: 14.919

3.  Analytical Description of Degradation-Relaxation Transformations in Nanoinhomogeneous Spinel Ceramics.

Authors:  O Shpotyuk; M Brunner; I Hadzaman; V Balitska; H Klym
Journal:  Nanoscale Res Lett       Date:  2016-11-14       Impact factor: 4.703

4.  Hard X-rays as pump and probe of atomic motion in oxide glasses.

Authors:  B Ruta; F Zontone; Y Chushkin; G Baldi; G Pintori; G Monaco; B Rufflé; W Kob
Journal:  Sci Rep       Date:  2017-06-21       Impact factor: 4.379

5.  On the use of two-time correlation functions for X-ray photon correlation spectroscopy data analysis.

Authors:  Oier Bikondoa
Journal:  J Appl Crystallogr       Date:  2017-02-17       Impact factor: 3.304

  5 in total

北京卡尤迪生物科技股份有限公司 © 2022-2023.