Literature DB >> 23002857

Adam-Gibbs relation for glass-forming liquids in two, three, and four dimensions.

Shiladitya Sengupta1, Smarajit Karmakar, Chandan Dasgupta, Srikanth Sastry.   

Abstract

The Adam-Gibbs relation between relaxation times and the configurational entropy has been tested extensively for glass formers using experimental data and computer simulation results. Although the form of the relation contains no dependence on the spatial dimensionality in the original formulation, subsequent derivations of the Adam-Gibbs relation allow for such a possibility. We test the Adam-Gibbs relation in two, three, and four spatial dimensions using computer simulations of model glass formers. We find that the relation is valid in three and four dimensions. But in two dimensions, the relation does not hold, and interestingly, no single alternate relation describes the results for the different model systems we study.

Year:  2012        PMID: 23002857     DOI: 10.1103/PhysRevLett.109.095705

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  8 in total

1.  Long-wavelength fluctuations and the glass transition in two dimensions and three dimensions.

Authors:  Skanda Vivek; Colm P Kelleher; Paul M Chaikin; Eric R Weeks
Journal:  Proc Natl Acad Sci U S A       Date:  2017-01-30       Impact factor: 11.205

2.  Power law relationship between diffusion coefficients in multi-component glass forming liquids.

Authors:  Anshul D S Parmar; Shiladitya Sengupta; Srikanth Sastry
Journal:  Eur Phys J E Soft Matter       Date:  2018-08-08       Impact factor: 1.890

3.  The relationship of dynamical heterogeneity to the Adam-Gibbs and random first-order transition theories of glass formation.

Authors:  Francis W Starr; Jack F Douglas; Srikanth Sastry
Journal:  J Chem Phys       Date:  2013-03-28       Impact factor: 3.488

4.  String-like cooperative motion in homogeneous melting.

Authors:  Hao Zhang; Mohammad Khalkhali; Qingxia Liu; Jack F Douglas
Journal:  J Chem Phys       Date:  2013-03-28       Impact factor: 3.488

5.  Dynamics of Glass Forming Liquids with Randomly Pinned Particles.

Authors:  Saurish Chakrabarty; Smarajit Karmakar; Chandan Dasgupta
Journal:  Sci Rep       Date:  2015-07-24       Impact factor: 4.379

6.  Apparent strength versus universality in glasses of soft compressible colloids.

Authors:  Ruben Higler; Joris Sprakel
Journal:  Sci Rep       Date:  2018-11-14       Impact factor: 4.379

7.  Zero-temperature glass transition in two dimensions.

Authors:  Ludovic Berthier; Patrick Charbonneau; Andrea Ninarello; Misaki Ozawa; Sho Yaida
Journal:  Nat Commun       Date:  2019-04-03       Impact factor: 14.919

Review 8.  Temperature Dependence of Structural Relaxation in Glass-Forming Liquids and Polymers.

Authors:  Vladimir N Novikov; Alexei P Sokolov
Journal:  Entropy (Basel)       Date:  2022-08-10       Impact factor: 2.738

  8 in total

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