Literature DB >> 22741915

Relativistic effects in photon-induced near field electron microscopy.

Sang Tae Park1, Ahmed H Zewail.   

Abstract

Electrons and photons, when interacting via a nanostructure, produce a new way of imaging in space and time, termed photon-induced near field electron microscopy or PINEM [Barwick et al. Nature 2009, 462, 902]. The phenomenon was described by considering the evanescent field produced by the nanostructure, but quantification of the experimental results was achieved by solving the Schrödinger equation for the interaction of the three bodies. The question remained, is the nonrelativistic formulation sufficient for this description? Here, relativistic and nonrelativistic quantum mechanical formulations are compared for electron-photon interaction mediated by nanostructures, and it is shown that there is an exact equivalence for the two formulations. The nonrelativistic formulation was found to be valid in the relativistic regime when using in the former formulation the relativistically corrected velocity (and the corresponding values of momentum and energy). In the PINEM experiment, 200 keV electrons were utilized, giving the experimental (relativistically corrected) velocity to be 0.7c(v without relativistic correction is 0.885c). When this value (0.7c), together with those of the corresponding momentum (p(c) = mv) and energy (E(c) = (1/2)mv(2)), is used in the first order solution of the Schrödinger formulation, an exact equivalence is obtained.

Mesh:

Year:  2012        PMID: 22741915     DOI: 10.1021/jp304534n

Source DB:  PubMed          Journal:  J Phys Chem A        ISSN: 1089-5639            Impact factor:   2.781


  5 in total

1.  Quantum coherent optical phase modulation in an ultrafast transmission electron microscope.

Authors:  Armin Feist; Katharina E Echternkamp; Jakob Schauss; Sergey V Yalunin; Sascha Schäfer; Claus Ropers
Journal:  Nature       Date:  2015-05-14       Impact factor: 49.962

2.  Graphene-layered steps and their fields visualized by 4D electron microscopy.

Authors:  Sang Tae Park; Aycan Yurtsever; John Spencer Baskin; Ahmed H Zewail
Journal:  Proc Natl Acad Sci U S A       Date:  2013-05-20       Impact factor: 11.205

3.  Quantum Effects In Imaging Nano-Structures Using Photon-Induced Near-Field Electron Microscopy.

Authors:  Naglaa Etman; Afaf M A Said; Khaled S R Atia; Reem Sultan; Mohamed Farhat O Hameed; Muhamed Amin; S S A Obayya
Journal:  Sci Rep       Date:  2019-04-16       Impact factor: 4.379

Review 4.  Optical Excitations with Electron Beams: Challenges and Opportunities.

Authors:  F Javier García de Abajo; Valerio Di Giulio
Journal:  ACS Photonics       Date:  2021-03-25       Impact factor: 7.529

5.  Modulation of Cathodoluminescence Emission by Interference with External Light.

Authors:  Valerio Di Giulio; Ofer Kfir; Claus Ropers; F Javier García de Abajo
Journal:  ACS Nano       Date:  2021-03-16       Impact factor: 15.881

  5 in total

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