Literature DB >> 22398557

Field-driven photoemission from nanostructures quenches the quiver motion.

G Herink1, D R Solli, M Gulde, C Ropers.   

Abstract

Strong-field physics, an extreme limit of light-matter interaction, is expanding into the realm of surfaces and nanostructures from its origin in atomic and molecular science. The attraction of nanostructures lies in two intimately connected features: local intensity enhancement and sub-wavelength confinement of optical fields. Local intensity enhancement facilitates access to the strong-field regime and has already sparked various applications, whereas spatial localization has the potential to generate strong-field dynamics exclusive to nanostructures. However, the observation of features unattainable in gaseous media is challenged by many-body effects and material damage, which arise under intense illumination of dense systems. Here, we non-destructively access this regime in the solid state by employing single plasmonic nanotips and few-cycle mid-infrared pulses, making use of the wavelength-dependence of the interaction, that is, the ponderomotive energy. We investigate strong-field photoelectron emission and acceleration from single nanostructures over a broad spectral range, and find kinetic energies of hundreds of electronvolts. We observe the transition to a new regime in strong-field dynamics, in which the electrons escape the nanolocalized field within a fraction of an optical half-cycle. The transition into this regime, characterized by a spatial adiabaticity parameter, would require relativistic electrons in the absence of nanostructures. These results establish new degrees of freedom for the manipulation and control of electron dynamics on femtosecond and attosecond timescales, combining optical near-fields and nanoscopic sources.

Year:  2012        PMID: 22398557     DOI: 10.1038/nature10878

Source DB:  PubMed          Journal:  Nature        ISSN: 0028-0836            Impact factor:   49.962


  17 in total

1.  Near-field second-harmonic generation induced by local field enhancement.

Authors:  A Bouhelier; M Beversluis; A Hartschuh; L Novotny
Journal:  Phys Rev Lett       Date:  2003-01-10       Impact factor: 9.161

2.  Origin of the high-energy electron emission from metals under laser irradiation.

Authors: 
Journal:  Phys Rev B Condens Matter       Date:  1992-06-01

3.  Generation of 0.4-keV femtosecond electron pulses using impulsively excited surface plasmons.

Authors:  S E Irvine; A Dechant; A Y Elezzabi
Journal:  Phys Rev Lett       Date:  2004-10-28       Impact factor: 9.161

4.  Isolated single-cycle attosecond pulses.

Authors:  G Sansone; E Benedetti; F Calegari; C Vozzi; L Avaldi; R Flammini; L Poletto; P Villoresi; C Altucci; R Velotta; S Stagira; S De Silvestri; M Nisoli
Journal:  Science       Date:  2006-10-20       Impact factor: 47.728

5.  Localized multiphoton emission of femtosecond electron pulses from metal nanotips.

Authors:  C Ropers; D R Solli; C P Schulz; C Lienau; T Elsaesser
Journal:  Phys Rev Lett       Date:  2007-01-25       Impact factor: 9.161

6.  High-harmonic generation by resonant plasmon field enhancement.

Authors:  Seungchul Kim; Jonghan Jin; Young-Jin Kim; In-Yong Park; Yunseok Kim; Seung-Woo Kim
Journal:  Nature       Date:  2008-06-05       Impact factor: 49.962

7.  Nanostructure-enhanced atomic line emission.

Authors:  M Sivis; M Duwe; B Abel; C Ropers
Journal:  Nature       Date:  2012-05-09       Impact factor: 49.962

8.  Terahertz near-field nanoscopy of mobile carriers in single semiconductor nanodevices.

Authors:  A J Huber; F Keilmann; J Wittborn; J Aizpurua; R Hillenbrand
Journal:  Nano Lett       Date:  2008-10-07       Impact factor: 11.189

9.  Strong-field above-threshold photoemission from sharp metal tips.

Authors:  Markus Schenk; Michael Krüger; Peter Hommelhoff
Journal:  Phys Rev Lett       Date:  2010-12-14       Impact factor: 9.161

10.  Tip-enhanced strong-field photoemission.

Authors:  R Bormann; M Gulde; A Weismann; S V Yalunin; C Ropers
Journal:  Phys Rev Lett       Date:  2010-09-27       Impact factor: 9.161

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  31 in total

Review 1.  Strong field transient manipulation of electronic states and bands.

Authors:  I Crassee; L Gallmann; G Gäumann; M Matthews; H Yanagisawa; T Feurer; M Hengsberger; U Keller; J Osterwalder; H J Wörner; J P Wolf
Journal:  Struct Dyn       Date:  2017-12-21       Impact factor: 2.920

2.  Quantum coherent optical phase modulation in an ultrafast transmission electron microscope.

Authors:  Armin Feist; Katharina E Echternkamp; Jakob Schauss; Sergey V Yalunin; Sascha Schäfer; Claus Ropers
Journal:  Nature       Date:  2015-05-14       Impact factor: 49.962

3.  Ultrafast strong-field photoemission from plasmonic nanoparticles.

Authors:  Péter Dombi; Anton Hörl; Péter Rácz; István Márton; Andreas Trügler; Joachim R Krenn; Ulrich Hohenester
Journal:  Nano Lett       Date:  2013-01-25       Impact factor: 11.189

4.  Strong-field plasmonic photoemission in the mid-IR at <1 GW/cm² intensity.

Authors:  S M Teichmann; P Rácz; M F Ciappina; J A Pérez-Hernández; A Thai; J Fekete; A Y Elezzabi; L Veisz; J Biegert; P Dombi
Journal:  Sci Rep       Date:  2015-01-12       Impact factor: 4.379

5.  Femtosecond few- to single-electron point-projection microscopy for nanoscale dynamic imaging.

Authors:  A R Bainbridge; C W Barlow Myers; W A Bryan
Journal:  Struct Dyn       Date:  2016-04-20       Impact factor: 2.920

6.  Photoemission-based microelectronic devices.

Authors:  Ebrahim Forati; Tyler J Dill; Andrea R Tao; Dan Sievenpiper
Journal:  Nat Commun       Date:  2016-11-04       Impact factor: 14.919

7.  Delayed electron emission in strong-field driven tunnelling from a metallic nanotip in the multi-electron regime.

Authors:  Hirofumi Yanagisawa; Sascha Schnepp; Christian Hafner; Matthias Hengsberger; Dong Eon Kim; Matthias F Kling; Alexandra Landsman; Lukas Gallmann; Jürg Osterwalder
Journal:  Sci Rep       Date:  2016-10-27       Impact factor: 4.379

8.  Field propagation-induced directionality of carrier-envelope phase-controlled photoemission from nanospheres.

Authors:  F Süßmann; L Seiffert; S Zherebtsov; V Mondes; J Stierle; M Arbeiter; J Plenge; P Rupp; C Peltz; A Kessel; S A Trushin; B Ahn; D Kim; C Graf; E Rühl; M F Kling; T Fennel
Journal:  Nat Commun       Date:  2015-08-12       Impact factor: 14.919

9.  Sub-phonon-period compression of electron pulses for atomic diffraction.

Authors:  A Gliserin; M Walbran; F Krausz; P Baum
Journal:  Nat Commun       Date:  2015-10-27       Impact factor: 14.919

10.  Ultrafast strong-field photoelectron emission from biased metal surfaces: exact solution to time-dependent Schrödinger Equation.

Authors:  Peng Zhang; Y Y Lau
Journal:  Sci Rep       Date:  2016-01-28       Impact factor: 4.379

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