Ekkehard Pomplun1. 1. Department of Safety and Radiation Protection, Forschungszentrum Jülich, D-52425 Jülich, Germany. e.pomplun@fz-juelich.de
Abstract
PURPOSE: To further validate Monte Carlo calculation codes simulating cascades of Auger electron transitions in radionuclides that decay by electron capture or internal conversion. In particular, the need for an appropriate kinetic energy determination of the Auger electrons emitted from multiple-ionized atoms as well as the consideration of shake-off electrons would be investigated implicitly. METHODS: Charge distributions of noble gases after photoionization for different photon energies were calculated and compared with experimental data from the literature. In addition, new electron emission spectra were generated for (99m)Tc and (123)I. RESULTS: By including strict energy book-keeping and allowing shake-off electrons, the agreement between experimentally detected charge distributions and Monte Carlo simulations was very good. On this basis, the number of emitted electrons per decay was found to be between 1 and 17 with a mean of 4.0 for (99m)Tc and between 1 and 26 with a mean of 7.4 for (123)I. CONCLUSIONS: Because of the good agreement with the experimental findings, the validation can be considered to be successful.
PURPOSE: To further validate Monte Carlo calculation codes simulating cascades of Auger electron transitions in radionuclides that decay by electron capture or internal conversion. In particular, the need for an appropriate kinetic energy determination of the Auger electrons emitted from multiple-ionized atoms as well as the consideration of shake-off electrons would be investigated implicitly. METHODS: Charge distributions of noble gases after photoionization for different photon energies were calculated and compared with experimental data from the literature. In addition, new electron emission spectra were generated for (99m)Tc and (123)I. RESULTS: By including strict energy book-keeping and allowing shake-off electrons, the agreement between experimentally detected charge distributions and Monte Carlo simulations was very good. On this basis, the number of emitted electrons per decay was found to be between 1 and 17 with a mean of 4.0 for (99m)Tc and between 1 and 26 with a mean of 7.4 for (123)I. CONCLUSIONS: Because of the good agreement with the experimental findings, the validation can be considered to be successful.
Authors: Mohammad Rezaee; Pierre Cloutier; Andrew D Bass; Marc Michaud; Darel J Hunting; Léon Sanche Journal: Phys Rev E Stat Nonlin Soft Matter Phys Date: 2012-09-14