Literature DB >> 21230079

Subdiffusion and intermittent dynamic fluctuations in the aging regime of concentrated hard spheres.

Djamel El Masri1, Ludovic Berthier, Luca Cipelletti.   

Abstract

We study the nonequilibrium aging dynamics in a system of quasihard spheres at large density by means of computer simulations. We find that, after a sudden quench to large density, the relaxation time initially increases exponentially with the age of the system. After a surprisingly large crossover time, the system enters the asymptotic aging regime characterized by a nearly linear increase in the relaxation time with age. In this aging regime, single-particle motion is strongly non-fickian, with a mean-squared displacement increasing subdiffusively, associated with broad non-gaussian tails in the distribution of particle displacements. We find that the system ages through temporally intermittent relaxation events, and a detailed finite-size analysis of these collective dynamic fluctuations reveals that these events are not spanning the entire system, but remain spatially localized.

Year:  2010        PMID: 21230079     DOI: 10.1103/PhysRevE.82.031503

Source DB:  PubMed          Journal:  Phys Rev E Stat Nonlin Soft Matter Phys        ISSN: 1539-3755


  2 in total

1.  Avalanches mediate crystallization in a hard-sphere glass.

Authors:  Eduardo Sanz; Chantal Valeriani; Emanuela Zaccarelli; Wilson C K Poon; Michael E Cates; Peter N Pusey
Journal:  Proc Natl Acad Sci U S A       Date:  2013-12-04       Impact factor: 11.205

2.  Common mechanism of thermodynamic and mechanical origin for ageing and crystallization of glasses.

Authors:  Taiki Yanagishima; John Russo; Hajime Tanaka
Journal:  Nat Commun       Date:  2017-06-29       Impact factor: 14.919

  2 in total

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