Literature DB >> 20871888

Simultaneous iridium catalysed oxidation and enzymatic reduction employing orthogonal reagents.

Francesco G Mutti1, Andreas Orthaber, Joerg H Schrittwieser, Johannes G de Vries, Rudolf Pietschnig, Wolfgang Kroutil.   

Abstract

An iridium catalysed oxidation was coupled concurrently to an asymmetric biocatalytic reduction in one-pot; thus it was shown for the first time that iridium- and alcohol dehydrogenase-catalysed redox reactions are compatible. As a model system racemic chlorohydrins were transformed to enantioenriched chlorohydrins via an oxidation-asymmetric reduction sequence.

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Year:  2010        PMID： 20871888     DOI： 10.1039/c0cc02813d

Source DB:  PubMed          Journal:  Chem Commun (Camb)        ISSN： 1359-7345            Impact factor:   6.222


  9 in total

1.  A supramolecular approach to combining enzymatic and transition metal catalysis.

Authors:  Z Jane Wang; Kristen N Clary; Robert G Bergman; Kenneth N Raymond; F Dean Toste
Journal:  Nat Chem       Date:  2013-01-06       Impact factor: 24.427

2.  Synthetic cascades are enabled by combining biocatalysts with artificial metalloenzymes.

Authors:  V Köhler; Y M Wilson; M Dürrenberger; D Ghislieri; E Churakova; T Quinto; L Knörr; D Häussinger; F Hollmann; N J Turner; T R Ward
Journal:  Nat Chem       Date:  2012-11-25       Impact factor: 24.427

Review 3.  Recent biocatalytic oxidation-reduction cascades.

Authors:  Joerg H Schrittwieser; Johann Sattler; Verena Resch; Francesco G Mutti; Wolfgang Kroutil
Journal:  Curr Opin Chem Biol       Date:  2010-12-02       Impact factor: 8.822

4.  Carbohydrate-Functionalized Triazolylidene Iridium Complexes: Hydrogenation Catalysis in Water with Asymmetric Induction.

Authors:  Joseph P Byrne; Lidia Delgado; Francesca Paradisi; Martin Albrecht
Journal:  ChemCatChem       Date:  2022-03-11       Impact factor: 5.497

5.  Synthesis of Enantiopure Sulfoxides by Concurrent Photocatalytic Oxidation and Biocatalytic Reduction.

Authors:  Sarah Bierbaumer; Luca Schmermund; Alexander List; Christoph K Winkler; Silvia M Glueck; Wolfgang Kroutil
Journal:  Angew Chem Int Ed Engl       Date:  2022-03-04       Impact factor: 16.823

6.  Synthesis of Optically Active syn- and anti-Chlorohydrins through a Bienzymatic Reductive Cascade.

Authors:  Jorge González-Rodríguez; Jesús Albarrán-Velo; Raquel G Soengas; Iván Lavandera; Vicente Gotor-Fernández; Humberto Rodríguez-Solla
Journal:  Org Lett       Date:  2022-09-26       Impact factor: 6.072

7.  Enantioselective synthesis of amines by combining photoredox and enzymatic catalysis in a cyclic reaction network.

Authors:  Xingwei Guo; Yasunori Okamoto; Mirjam R Schreier; Thomas R Ward; Oliver S Wenger
Journal:  Chem Sci       Date:  2018-05-17       Impact factor: 9.825

Review 8.  Biocatalytic Reduction Reactions from a Chemist's Perspective.

Authors:  Frank Hollmann; Diederik J Opperman; Caroline E Paul
Journal:  Angew Chem Int Ed Engl       Date:  2020-11-03       Impact factor: 15.336

9.  Chemoenzymatic Asymmetric Synthesis of Pyridine-Based α-Fluorinated Secondary Alcohols.

Authors:  Timo Broese; Peter Ehlers; Peter Langer; Jan von Langermann
Journal:  Chembiochem       Date:  2021-10-07       Impact factor: 3.461
  9 in total

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