| Literature DB >> 20721156 |
Mark E Siemens1, Galan Moody, Hebin Li, Alan D Bristow, Steven T Cundiff.
Abstract
We derive an analytical form for resonance lineshapes in two-dimensional (2D) Fourier transform spectroscopy. Our starting point is the solution of the optical Bloch equations for a two-level system in the 2D time domain. Application of the projection-slice theorem of 2D Fourier transforms reveals the form of diagonal and cross-diagonal slices in the 2D frequency data for arbitrary inhomogeneity. The results are applied in quantitative measurements of homogeneous and inhomogeneous broadening of multiple resonances in experimental data.Mesh:
Year: 2010 PMID: 20721156 DOI: 10.1364/OE.18.017699
Source DB: PubMed Journal: Opt Express ISSN: 1094-4087 Impact factor: 3.894